NDLI: Research on the optical spectra, g factors and defect structures for two tetragonal Y²+ centers in the irradiated CaF2: Y crystal.

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Research on the optical spectra, g factors and defect structures for two tetragonal Y²+ centers in the irradiated CaF2: Y crystal.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Zheng, Wen-Chen Yang, Yu-Guang Mei, Yang Liu, Hong-Gang
Description	Author Affiliation: Zheng WC ( Department of Material Science, Sichuan University, Chengdu 610064, PR China. zhengwc1@163.com)
Abstract	Based on the defect models that the tetragonal Y(2+) (1) center in the irradiated CaF(2): Y crystal is due to Y(2+) at Ca(2+) site associated with a nearest interstitial F(-) ion along C(4) axis and the tetragonal Y(2+) (2) center is Y(2+) at Ca(2+) site where the tetragonal distortion is caused by the static Jahn-Teller effect, the two optical spectral bands and anisotropic g factors for both tetragonal Y(2+) centers are calculated. The calculations are made by using two methods based on the cluster approach, one is the complete diagonalization (of energy matrix) method (CDM) and another is the perturbation theory method (PTM). The calculated results for each Y(2+) center from CDM and PTM coincide and show reasonable agreement with the experimental values. The calculated isotropic g factor for Y(2+) (2) center at higher temperature owing to the dynamical Jahn-Teller effect is also consistent with the observed value. The defect structures (i.e., tetragonal distortion) of the two Y(2+) centers are obtained from the calculation. It appears that both theoretical methods can be applied to explain the optical and EPR data, to study the defect model and to determine the defect structures for d(1) ions in crystals.
ISSN	13861425
Journal	Spectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy
Volume Number	97
e-ISSN	18733557
Language	English
Publisher	Elsevier
Publisher Date	2012-11-01
Publisher Place	Great Britain (UK)
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Calcium Fluoride Chemistry Optical Phenomena Crystallization Electron Spin Resonance Spectroscopy Ions Journal Article Discipline Spectroscopy
Content Type	Text
Resource Type	Article
Subject	Spectroscopy Atomic and Molecular Physics, and Optics Analytical Chemistry Instrumentation

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