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A natural carbonized leaf as polysulfide diffusion inhibitor for high-performance lithium-sulfur battery cells.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Chung, Sheng-Heng Manthiram, Arumugam
Description	Author Affiliation: Chung SH ( Electrochemical Energy Laboratory & Materials Science and Engineering Program, The University of Texas at Austin, Austin, TX 78712 (USA).)
Abstract	Attracted by the unique tissue and functions of leaves, a natural carbonized leaf (CL) is presented as a polysulfide diffusion inhibitor in lithium-sulfur (Li-S) batteries. The CL that is covered on the pure sulfur cathode effectively suppresses the polysulfide shuttling mechanism and enables the use of pure sulfur as the cathode. A low charge resistance and a high discharge capacity of 1320âmA h g(-1) arise from the improved cell conductivity due to the innately integral conductive carbon network of the CL. The unique microstructure of CL leads to a high discharge/charge efficiency of >98 %, low capacity fade of 0.18 % per cycle, and good long-term cyclability over 150âcycles. The structural gradient and the micro/mesoporous adsorption sites of CL effectively intercept/trap the migrating polysulfides and facilitate their reutilization. The green CL polysulfide diffusion inhibitor thus offers a viable approach for developing high-performance lithium-sulfur batteries.
File Format	HTM / HTML
ISSN	18645631
Issue Number	6
Volume Number	7
e-ISSN	1864564X
Journal	ChemSusChem
Language	English
Publisher	Wiley-VCH
Publisher Date	2014-06-01
Publisher Place	Germany
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Electric Power Supplies Sulfides Green Chemistry Technology Research Support, Non-u.s. Gov't Chemistry Plant Leaves Discipline Sustainable Chemistry Lithium Diffusion Sulfur Carbon Journal Article
Content Type	Text
Resource Type	Article
Subject	Energy Environmental Chemistry Materials Science Chemical Engineering

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A natural carbonized leaf as polysulfide diffusion inhibitor for high-performance lithium-sulfur battery cells.

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