NDLI: Ionic-liquid-assisted synthesis of nanostructured and carbon-coated Li3V2(PO4)3 for high-power electrochemical storage devices.

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Ionic-liquid-assisted synthesis of nanostructured and carbon-coated Li3V2(PO4)3 for high-power electrochemical storage devices.

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Ionic-liquid-assisted synthesis of nanostructured and carbon-coated Li3V2(PO4)3 for high-power electrochemical storage devices.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Zhang, Xiaofei Böckenfeld, Nils Berkemeier, Frank Balducci, Andrea
Description	Author Affiliation: Zhang X ( Westfälische Wilhelms Universität, Institut für Physikalische Chemie-MEET, Corrensstrasse 28/30, 48149 Münster (Germany).)
Abstract	Carbon-coated Li3V2(PO4)3 (LVP) displaying nanostructured morphology can be easily prepared by using ionic-liquid-assisted sol-gel synthesis. The selection of highly viscous and thermally stable ionic liquids might promote the formation of nanostructures during the sol-gel synthesis. The presence of these structures shortens the diffusion paths and enlarges the contact area between the active material and the electrolyte; this leads to a significant improvement in lithium-ion diffusion. At the same time, the use of ionic liquids has a positive influence on the coating of the LVP particles, which improves the electronic conductivity of this material; this leads to enhanced charge-transfer properties. At a high current density of 40âC, the LVP/N-butyl-N-methylpyrrolidinium bis(trifluoromethanesulfonyl)imide material delivered a reversible capacity of approximately 100âmA h g(-1), and approximately 99 % of the initial capacity value was retained even after 100âcycles at 50âC. The excellent high rate and cycling stability performance make Li3V2(PO4)3 prepared by ionic-liquid-assisted sol-gel synthesis a very promising cathode material for high-power electrochemical storage devices.
File Format	HTM / HTML
ISSN	18645631
Issue Number	6
Volume Number	7
e-ISSN	1864564X
Journal	ChemSusChem
Language	English
Publisher	Wiley-VCH
Publisher Date	2014-06-01
Publisher Place	Germany
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Phosphates Ionic Liquids Electric Power Supplies Research Support, Non-u.s. Gov't Discipline Sustainable Chemistry Lithium Nanostructures Carbon Journal Article Vanadium Compounds Chemistry Imidazoles Sulfonamides Electrochemistry Dielectric Spectroscopy
Content Type	Text
Resource Type	Article
Subject	Energy Environmental Chemistry Materials Science Chemical Engineering

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