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| Content Provider | IEEE Xplore Digital Library |
|---|---|
| Author | Lang, P. Homann, C. Pugliesi, I. Kienberger, R. Riedle, E. |
| Copyright Year | 2011 |
| Description | Author affiliation: Department für Physik, TU München, Germany (Kienberger, R.) || Lehrstuhl für BioMolekulare Optik, LMU München, Germany (Lang, P.; Homann, C.; Pugliesi, I.; Riedle, E.) |
| Abstract | Time resolved photoelectron spectroscopy is a versatile tool for the investigation of ultrafast dynamics in optically dark regions of the molecular potential energy surface. We developed a novel pump-probe-setup, which consists of a magnetic bottle spectrometer and two tunable laser pulses with pulse durations better than 30fs. The pump pulse covers a range of 240 – 400 nm due to frequency doubling of a NOPA and is used to excite the molecules. The temporally delayed probe pulse with 200 – 240 nm tunability ionizes the excited molecules and is generated by sum frequency mixing the frequency doubled output of a second NOPA with a part of the fundamental Ti:sapphire laser pulse. This deep-UV probe pulse samples a large range of the electron kinetic energy spectrum up to 3 eV. The tunability allows us to minimize the contribution of electronic excitations by the probe pulse alone. To achieve pulses with a minimum chirp in the interaction zone we are using prism compressors after each NOPA to give the pulse a positive chirp. |
| Starting Page | 1 |
| Ending Page | 1 |
| File Size | 351150 |
| Page Count | 1 |
| File Format | |
| ISBN | 9781457705335 |
| e-ISBN | 9781457705328 |
| DOI | 10.1109/CLEOE.2011.5943524 |
| Language | English |
| Publisher | Institute of Electrical and Electronics Engineers, Inc. (IEEE) |
| Publisher Date | 2011-05-22 |
| Publisher Place | Germany |
| Access Restriction | Subscribed |
| Rights Holder | Institute of Electrical and Electronics Engineers, Inc. (IEEE) |
| Subject Keyword | Irrigation Optical pumping Probes |
| Content Type | Text |
| Resource Type | Article |
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