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| Content Provider | IEEE Xplore Digital Library |
|---|---|
| Author | Croce, M.P. Bond, E.M. Hoover, A.S. Kunde, G.J. Mocko, V. Rabin, M. Weisse-Bernstein, N.R. Wolfsberg, L.E. Bennett, D.A. Hays-Wehle, J. Schmidt, D.R. Ullom, J.N. |
| Copyright Year | 2002 |
| Abstract | We discuss sensor and method development for the analysis of alphaand beta-decaying radioisotopes encapsulated within superconducting transition-edge sensor microcalorimeter absorbers. For alpha-decaying isotopes, e.g., 238Pu, 241Am, and 210Po, this is a measurement of the total nuclear reaction energy (Q) and the spectra consist of sharp, narrow peaks. The primary peak is at the Q value, with secondary peaks corresponding to gamma-ray-escape peaks. In contrast, for beta-decaying isotopes, e.g., 241Pu, the spectrum is a low energy continuum ending at E=Q. We are developing transition edge-sensor (TES) microcalorimeters to measure these spectra simultaneously in a single sample, hence allowing quantitative analysis of all Pu isotopes from 238 to 242. We have developed and used TES microcalorimeter detectors for this purpose, and it represents a new quantitative analysis tool for nuclear forensics and safeguards. Due to the high efficiency of the embedded source geometry, measurement times can be minimized. The high dynamic range of our sensors creates the opportunity to measure the relatively low energy beta-decay spectrum of 241Pu (Q = 20.78 keV) simultaneously with the Q ~ 5-6 MeV of alpha-decaying actinides. Finally, the technique could also be effective for determining the time since chemical purification of Pu using the 241Pu/241Am isotopic ratio via simultaneous measurement of the low-energy 241Pu beta particles and the high-energy 241Am Q-value. |
| Sponsorship | Council on Superconductivity Appl. Superconductivity Conference Inc MIT |
| Starting Page | 1 |
| Ending Page | 3 |
| Page Count | 3 |
| File Size | 550054 |
| File Format | |
| ISSN | 10518223 |
| Volume Number | 25 |
| Issue Number | 3 |
| Language | English |
| Publisher | Institute of Electrical and Electronics Engineers, Inc. (IEEE) |
| Publisher Date | 2015-01-01 |
| Publisher Place | U.S.A. |
| Access Restriction | One Nation One Subscription (ONOS) |
| Rights Holder | Institute of Electrical and Electronics Engineers, Inc. (IEEE) |
| Subject Keyword | Detectors Energy measurement Isotopes Spectroscopy Dynamic range Chemicals Data acquisition transition-edge sensor microcalorimeter nuclear forensics transition-edge sensor (TES) Microcalorimeter Q-spectroscopy |
| Content Type | Text |
| Resource Type | Article |
| Subject | Condensed Matter Physics Electronic, Optical and Magnetic Materials Electrical and Electronic Engineering |
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