NDLI: Mn/Ti-doped carbon xerogel for efficient catalysis of microcystin-LR degradation in the water surface discharge plasma reactor.

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Mn/Ti-doped carbon xerogel for efficient catalysis of microcystin-LR degradation in the water surface discharge plasma reactor.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Zhang, Yi Lei, Lecheng Yang, Bin Li, Zhongjian Xin, Qing
Description	Country affiliation: China Author Affiliation: Xin Q ( Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, 310027, China.); Zhang Y ( College of Electronic Information, Hangzhou Dianzi University, Hangzhou, 310018, China.); Li Z ( School of Environmental Science and Engineering, Zhejiang Gongshang University, Hangzhou, 310012, Zhejiang, People's Republic of China.); Lei L ( Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, 310027, China.); Yang B ( Key Laboratory of Biomass Chemical Engineering of Ministry of Education, College of Chemical and Biological Engineering, Zhejiang University, Hangzhou, 310027, China.)
Abstract	The novel catalysts of Mn/Ti-doped carbon xerogel (CX) were synthesized for efficient degradation of microcystin-LR (MC-LR) in the water surface discharge plasma reactor. The degradation efficiency of 79.7% was obtained in 6 min with 0.5 wt% Ti impregnation of CX, and it would be increased with higher amount of Ti. In particular, Mn-doped CX resulted in larger mesoporous particle diameter and higher porosity in the matrix, and thereby, the highest efficiency of 88.6% was achieved for CX-Ti-Mn. The possible degradation pathway of MC-LR was elucidated on the basis of the LC-MS analysis. It demonstrated that Adda chain was cleaved from the MC-LR cyclic peptide by OH radical attack after plasma discharge in the presence of catalysts, and the generated nontoxic products can be further easily degraded in the biological treatment. Therefore, Mn/Ti-doped carbon xerogel is promising as the catalyst for the improvement of MC-LR degradation in the water surface discharge plasma reactor.
ISSN	09441344
Issue Number	21
Volume Number	22
e-ISSN	16147499
Journal	Environmental Science and Pollution Research
Language	English
Publisher	Springer
Publisher Date	2015-11-01
Publisher Place	Germany
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Carbon Chemistry Manganese Microcystins Analysis Titanium Water Pollutants, Chemical Water Purification Methods Catalysis Gels Mass Spectrometry Porosity Surface Properties Ultraviolet Rays Journal Article Research Support, Non-u.s. Gov't Discipline Environmental Science Discipline Environmental Chemistry
Content Type	Text
Resource Type	Article
Subject	Environmental Chemistry Health, Toxicology and Mutagenesis Pollution Medicine

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