NDLI: Triazine-Based Polymers as Nanostructured Supports for the Liquid-Phase Oxidation of Alcohols

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Triazine-Based Polymers as Nanostructured Supports for the Liquid-Phase Oxidation of Alcohols

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Triazine-Based Polymers as Nanostructured Supports for the Liquid-Phase Oxidation of Alcohols

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Prati, Laura Villa, Alberto Thomas, Arne Chan-thaw, Carine E.
Description	Author Affiliation: Chan-Thaw CE ( Department of Chemistry, Functional Materials, Technische Universität Berlin, Englische Str. 20, 10587 Berlin, Germany.)
Abstract	A covalent triazine framework (CTF) was used as support for palladium nanoparticles (NPs) and Pd/CTF was applied as the catalyst in the selective oxidation of benzyl alcohol. N groups in the CTF appeared more efficient than those created on carbon nanotubes (CNTs) by $NH_{3}/high-temperature$ treatment in stabilizing Pd NPs against growth during the immobilization step. This assured a high metal dispersion, which led to a highly active and stable catalyst in the alcohol oxidation reaction. Indeed, Pd on the CTF was more stable in recycling than Pd on activated carbon (AC) and on nitrogen-doped CNTs, particularly avoiding leaching of Pd NPs. Moreover, Pd on the CTF was less sensitive than Pd on AC to the decrease of reactant concentration. This in turn led to a higher selectivity to benzaldehyde (98 %) with a considerable activity (turnover frequency $1453 h^{−1}).$
ISSN	09476539
e-ISSN	15213765
Journal	Chemistry - A European Journal
Issue Number	3
Volume Number	17
Language	English
Publisher	Wiley-VCH;ChemPubSoc Europe
Publisher Date	2011-01-17
Publisher Place	Germany
Access Restriction	Open
Subject Keyword	Chemistry
Content Type	Text
Resource Type	Article
Subject	Organic Chemistry Catalysis

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