NDLI: Applications of metal-organic frameworks in heterogeneous supramolecular catalysis.

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Applications of metal-organic frameworks in heterogeneous supramolecular catalysis.

Content Provider	Semantic Scholar
Author	Liu, Jiewei Chen, Lianfen Cui, Hao Zhang, Jianyong Zhang, Li Su, Cheng-Yong
Copyright Year	2014
Abstract	This review summarizes the use of metal-organic frameworks (MOFs) as a versatile supramolecular platform to develop heterogeneous catalysts for a variety of organic reactions, especially for liquid-phase reactions. Following a background introduction about catalytic relevance to various metal-organic materials, crystal engineering of MOFs, characterization and evaluation methods of MOF catalysis, we categorize catalytic MOFs based on the types of active sites, including coordinatively unsaturated metal sites (CUMs), metalloligands, functional organic sites (FOS), as well as metal nanoparticles (MNPs) embedded in the cavities. Throughout the review, we emphasize the incidental or deliberate formation of active sites, the stability, heterogeneity and shape/size selectivity for MOF catalysis. Finally, we briefly introduce their relevance into photo- and biomimetic catalysis, and compare MOFs with other typical porous solids such as zeolites and mesoporous silica with regard to their different attributes, and provide our view on future trends and developments in MOF-based catalysis.
Starting Page	455
Ending Page	461
Page Count	7
File Format	PDF HTM / HTML
Alternate Webpage(s)	http://pubs.rsc.org/en/content/getauthorversionpdf/C4CS00094C
PubMed reference number	24871268v1
Alternate Webpage(s)	https://doi.org/10.1039/c4cs00094c
DOI	10.1039/c4cs00094c
Journal	Chemical Society reviews
Volume Number	43
Issue Number	16
Language	English
Access Restriction	Open
Subject Keyword	Biomimetics Catalysis Embedding Genetic Heterogeneity Metal Nanoparticles Silicic Acid Solute Carrier Organic Anion Transporter Family Member 1b1 Zeolites solid substance
Content Type	Text
Resource Type	Article

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