NDLI: Sub-100 nm wrinkling of polydimethylsiloxane by double frontal oxidation

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Recent progress in cellulose nanocrystals: sources and production

Titania-coated gold nanorods with expanded photocatalytic response. Enzyme-like glucose oxidation under near-infrared illumination

Spatially uniform resistance switching of low current, high endurance titanium–niobium-oxide memristors

Spontaneous decoration of silicon surfaces with MoO_x nanoparticles for the sunlight-assisted hydrogen evolution reaction

B₄₀ cluster stability, reactivity, and its planar structural precursor

Janus PEGylated gold nanoparticles: a robust colorimetric probe for sensing nitrite ions in complex samples

Bimetallic catalytic growth of boron nitride nanotubes

Tunable UV-visible absorption of SnS₂ layered quantum dots produced by liquid phase exfoliation

Transfer-free multi-layer graphene as a diffusion barrier

Rh nanoparticles supported on ultrathin carbon nanosheets for high-performance oxygen reduction reaction and catalytic hydrogenation

The timeline of corona formation around silica nanocarriers highlights the role of the protein interactome

Paper microchip with a graphene-modified silver nano-composite electrode for electrical sensing of microbial pathogens

The supercoiling state of DNA determines the handedness of both H3 and CENP-A nucleosomes

Large-area tungsten disulfide for ultrafast photonics

Complete ultrafast charge carrier dynamics in photo-excited all-inorganic perovskite nanocrystals (CsPbX₃)

Advantages of an optical nanosensor system for the mechanistic analysis of a novel topoisomerase I targeting drug: a case study

Order of magnitude improvement of nano-contact spin torque nano-oscillator performance

Nanostructuration of ionic liquids: impact on the cation mobility. A multi-scale study

Excitation wavelength independent visible color emission of carbon dots

Highly sensitive and fast monolayer WS₂ phototransistors realized by SnS nanosheet decoration

Naked eye plasmonic indicator with multi-responsive polymer brush as signal transducer and amplifier

A core–multiple shell nanostructure enabling concurrent upconversion and quantum cutting for photon management

Carbon/two-dimensional MoTe₂ core/shell-structured microspheres as an anode material for Na-ion batteries

Real-time monitoring of plasmon induced dissociative electron transfer to the potential DNA radiosensitizer 8-bromoadenine

Spontaneous assembly of a hybrid crystal-liquid phase in inverse patchy colloid systems

Revisiting the optimized doping ratio in core/shell nanostructured upconversion particles

Bottom-up synthesis of nitrogen-doped porous carbon scaffolds for lithium and sodium storage

A dual-scale metal nanowire network transparent conductor for highly efficient and flexible organic light emitting diodes

A colorimetric sensing platform based upon recognizing hybridization chain reaction products with oligonucleotide modified gold nanoparticles through triplex formation

Co-immobilization of glucose oxidase and catalase for enhancing the performance of a membraneless glucose biofuel cell operated under physiological conditions

Imparting surface hydrophobicity to metal–organic frameworks using a facile solution-immersion process to enhance water stability for CO₂ capture

Bright conjugated polymer nanoparticles containing a biodegradable shell produced at high yields and with tuneable optical properties by a scalable microfluidic device

MoO_3−x quantum dots for photoacoustic imaging guided photothermal/photodynamic cancer treatment

Sub-100 nm wrinkling of polydimethylsiloxane by double frontal oxidation

3D printable conducting hydrogels containing chemically converted graphene

Au@Ag SERRS tags coupled to a lateral flow immunoassay for the sensitive detection of pneumolysin

Three-dimensional nano-heterojunction networks: a highly performing structure for fast visible-blind UV photodetectors

General criterion to distinguish between Schottky and Ohmic contacts at the metal/two-dimensional semiconductor interface

Titanocene dichloride (Cp₂TiCl₂) as a precursor for template-free fabrication of hollow TiO₂ nanostructures with enhanced photocatalytic hydrogen production

Energy transfer and depolarization in the photoluminescence of a plasmonic molecule

Effect of the solvent used for fabrication of perovskite films by solvent dropping on performance of perovskite light-emitting diodes

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Sub-100 nm wrinkling of polydimethylsiloxane by double frontal oxidation

Content Provider	Royal Society of Chemistry (RSC)
Author	Foglia, Fabrizia Cabral, João T. Matar, Omar K. Nania, Manuela
Copyright Year	2017
Abstract	We demonstrate nanoscale wrinkling on polydimethylsiloxane (PDMS) at sub-100 nm length scales via a (double) frontal surface oxidation coupled with a mechanical compression. The kinetics of the glassy skin propagation is resolved by neutron and X-ray reflectivity, and atomic force microscopy, combined with mechanical wrinkling experiments to evaluate the resulting pattern formation. In conventional PDMS surface oxidation, the smallest wrinkling patterns attainable have an intrinsic lower wavelength limit due to the coupling of skin formation and front propagation at fixed strain εprestrain, whose maximum is, in turn, set by material failure. However, combining two different oxidative processes, ultra-violet ozonolysis followed by air plasma exposure, we break this limit by fabricating trilayer laminates with excellent interfacial properties and a sequence of moduli and layer thicknesses able to trivially reduce the surface topography to sub-100 nm dimensions. This method provides a powerful, yet simple, non-lithographic approach to extend surface patterning from visible to the deep UV range.
Starting Page	2030
Ending Page	2037
Page Count	8
File Format	HTM / HTML PDF
ISSN	20403364
Volume Number	9
Issue Number	5
Journal	Nanoscale
DOI	10.1039/c6nr08255f
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Ozonolysis Pattern formation Atomic-force microscopy Cell membrane X-ray reflectivity Polydimethylsiloxane Neutron Wavelength
Content Type	Text
Resource Type	Article
Subject	Nanoscience and Nanotechnology

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Supporting Information Sub-100 nm wrinkling of polydimethylsiloxane by double surface oxidation

Oxidation of ultrathin GaSe

Polymer nanotubules obtained by layer-by-layer deposition within AAO-membrane templates with sub-100-nm pore diameters.

Scanned Probe Oxidation onp-GaAs(100) Surface with an Atomic Force Microscopy

Towards sub-100-nm X-ray microscopy for tomographic applications

Towards sub-100 nm x-ray microscopy for tomographic applications.

Orthoclase surface structure dissolution measured in situ by x-ray reflectivity and atomic force microscopy.

Sub-38 nm resolution microscopy with a tabletop 13 nm wavelength laser

Dynamic Structural Change of Plant Epidermal Cell Walls under Strain

Sub-100 nm wrinkling of polydimethylsiloxane by double frontal oxidation

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Supporting Information Sub-100 nm wrinkling of polydimethylsiloxane by double surface oxidation

Oxidation of ultrathin GaSe

Polymer nanotubules obtained by layer-by-layer deposition within AAO-membrane templates with sub-100-nm pore diameters.

Scanned Probe Oxidation onp-GaAs(100) Surface with an Atomic Force Microscopy

Towards sub-100-nm X-ray microscopy for tomographic applications

Towards sub-100 nm x-ray microscopy for tomographic applications.

Orthoclase surface structure dissolution measured in situ by x-ray reflectivity and atomic force microscopy.

Sub-38 nm resolution microscopy with a tabletop 13 nm wavelength laser

Dynamic Structural Change of Plant Epidermal Cell Walls under Strain

Sub-100 nm wrinkling of polydimethylsiloxane by double frontal oxidation