NDLI: Facile chemical solution synthesis of p-type delafossite Ag-based transparent conducting AgCrO<sub>2</sub> films in an open condition

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Journal of Materials Chemistry C Vol - 5 Issue - 7

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Facile chemical solution synthesis of p-type delafossite Ag-based transparent conducting AgCrO₂ films in an open condition

Content Provider	Royal Society of Chemistry (RSC)
Author	Sun, Yuping Tang, Xianwu Zhu, Xuebin Song, Wenhai Dai, Jianming Wei, Renhuai Yang, Jie Zhu, Xiaoguang Hu, Ling
Copyright Year	2017
Abstract	Recent progress in transparent conducting components stimulates the extensive exploration of p-type transparent conducting oxide (TCO) materials. Here, we report the synthesis of a class of p-type delafossite Ag-based TCO thin films, AgCrO2 (ACO), using a facile chemical solution route in an open condition. Firstly, the evolution of microstructure, morphology, and optical properties with respect to annealing temperature is reported. The stoichiometric ACO thin films show self-assembled c-axis orientation. The 500 °C-annealed ACO thin film presents a relatively high quality, dense surface and good optical transmittance amongst all the derived thin films. Then, to improve the conductivity, Mg doping effects are investigated. Upon Mg doping, p-type conductivity is obtained for thin films of AgCr1−xMgxO2 (0.04 ≤ x ≤ 0.20). The conductivity initially increases from 3.1 × 10−3 to 67.7 × 10−3 S cm−1 with x increasing from 0.04 to 0.12 and then slightly decreases with further increasing Mg concentration. The Hall results display that the hole concentration gradually increases with increasing Mg dopant concentration, and the carrier mobility first increases with x increasing from 0.04 to 0.12, while decreases with x further increasing from 0.12 to 0.20. A high magnitude of optical transmittance near 60% in the visible region and wide optical bandgaps (3.41–3.66 eV) of the AgCr1−xMgxO2 thin films are observed. The facial fabrication of ACO thin films in an open condition will provide a start for the synthesis of Ag-based delafossite thin films.
Starting Page	1885
Ending Page	1892
Page Count	8
File Format	HTM / HTML PDF
ISSN	20507526
Volume Number	5
Issue Number	8
Journal	Journal of Materials Chemistry C
DOI	10.1039/c6tc04848j
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	TCO Extrinsic semiconductor Transparent conducting film Automobile Club de l'Ouest Nucleic acid thermodynamics Stoichiometry Dopant Electronvolt
Content Type	Text
Resource Type	Article
Subject	Chemistry Materials Chemistry

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Facile chemical solution synthesis of p-type delafossite Ag-based transparent conducting AgCrO₂ films in an open condition

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Facile chemical solution synthesis of p-type delafossite Ag-based transparent conducting AgCrO₂ films in an open condition