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| Content Provider | IEEE Xplore Digital Library |
|---|---|
| Author | Wang, J.L. Studer, A.J. Campbell, S.J. Kennedy, S.J. Zeng, R. Dou, S.X. Wu, G.H. |
| Copyright Year | 1965 |
| Abstract | The magnetic structures of Pr0.8Lu0.2Mn2Ge2 and Pr0.6Lu0.4Mn2Ge2 have been determined by neutron powder diffraction over the temperature range 10-450 K. On cooling from the paramagnetic region the Mn sublattice of Pr0.8Lu0.2Mn2Ge2 orders in a similar manner to PrMn2Ge2 with first ab-plane intralayer antiferromagnetism (AFl) below TNintra ~ 397 K followed by canted ferromagnetism (Fmc) at TCinter ~ 330 K and then a conical (Fmi) spin structure below Tc/c ~ 192 K. The transition at TCPr=35 K with related enhancement in magnetization, is assigned to the additional ferromagnetic contribution of the Pr sublattice leading to the combined (Fmc+F(Pr)). For Pr0.6Lu0.4Mn2Ge2 the transition from PM to AFl occurs at TNintra ~ 375 K while the canted ferromagnetic (Fmc) state forms at TCinter ~ 321 K . The increased Lu concentration of Pr0.6Lu0.4Mn2Ge2 destroys the incommensurate Fmi conical spin structure of Pr0.8Lu0.2Mn2Ge2. Rather, in common with similar mixed RT2X2 systems (e.g., La1-xYxMn2Si2, La1-xPrxMn2Si2), the Pr0.6Lu0.4Mn2Ge2 compound exhibits co-existence of the AFmc and Fmc phases on cooling from the pure Fmc state. Transformation to the combined ferromagnetic state (Fmc+F(Pr)) takes place on c-axis ordering of the Pr sublattice at TCPr ~ 31 K . In the region of phase co-existence, the Fmc unit cell is larger than the AFmc unit cell indicating strong magneto-structural coupling with a change of the lattice inducing a change of the magnetic state. |
| Sponsorship | IEEE Magnetics Society |
| Starting Page | 2893 |
| Ending Page | 2896 |
| Page Count | 4 |
| File Size | 798977 |
| File Format | |
| ISSN | 00189464 |
| Volume Number | 47 |
| Issue Number | 10 |
| Language | English |
| Publisher | Institute of Electrical and Electronics Engineers, Inc. (IEEE) |
| Publisher Date | 2011-10-01 |
| Publisher Place | U.S.A. |
| Access Restriction | One Nation One Subscription (ONOS) |
| Rights Holder | Institute of Electrical and Electronics Engineers, Inc. (IEEE) |
| Subject Keyword | Manganese Diffraction Magnetic resonance imaging Neutrons Temperature distribution Perpendicular magnetic anisotropy rare earth transition metal compounds Magnetic phase transition magnetic structure neutron diffraction |
| Content Type | Text |
| Resource Type | Article |
| Subject | Electronic, Optical and Magnetic Materials Electrical and Electronic Engineering |
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