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| Content Provider | The American Society of Mechanical Engineers (ASME) Digital Collection |
|---|---|
| Author | Partha, P. Mukherjee Mukundan, Rangachary Rodney, L. Borup |
| Copyright Year | 2010 |
| Abstract | The gas diffusion layer (GDL) plays a critical role in the overall performance of a polymer electrolyte fuel cell (PEFC), especially in the mass transport control regime due to suboptimal liquid water transport. Liquid water blocks the porous pathways in the catalyst layer and gas diffusion layer thereby causing hindered oxygen transport from the channel to the active reaction sites. This phenomenon is known as “flooding” and is perceived as the primary mechanism leading to the limiting current behavior in the cell performance. The pore morphology and wetting characteristics of the cathode GDL are of paramount importance in the effective PEFC water management. Typical beginning-of-life GDLs exhibit hydrophobic characteristics, which facilities liquid water transport and hence reduces flooding. Experimental data, however, suggest that the GDL loses hydrophobicity over prolonged PEFC operation and becomes prone to enhanced flooding. In this work, we present a pore-scale modeling framework to study the structure-wettability-durability interplay in the context of flooding behavior in the PEFC GDL. |
| Sponsorship | Advanced Energy Systems Division |
| Starting Page | 683 |
| Ending Page | 688 |
| Page Count | 6 |
| File Format | |
| ISBN | 9780791844045 |
| DOI | 10.1115/FuelCell2010-33241 |
| e-ISBN | 9780791838754 |
| Volume Number | ASME 2010 8th International Fuel Cell Science, Engineering and Technology Conference: Volume 1 |
| Conference Proceedings | ASME 2010 8th International Conference on Fuel Cell Science, Engineering and Technology |
| Language | English |
| Publisher Date | 2010-06-14 |
| Publisher Place | Brooklyn, New York, USA |
| Access Restriction | Subscribed |
| Subject Keyword | Water Oxygen Catalysts Wetting Water resource management Durability Hydrophobicity Floods Modeling Fuel cells Gas diffusion layers Electrolytes Polymers |
| Content Type | Text |
| Resource Type | Article |
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