NDLI: Monitoring of hexabromocyclododecane diastereomers in fish from European freshwaters and estuaries.

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Monitoring of hexabromocyclododecane diastereomers in fish from European freshwaters and estuaries.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Klein, Roland Rüdel, Heinz Müller, Josef Quack, Markus
Spatial Coverage	Europe
Description	Country affiliation: Germany Author Affiliation: Rüdel H ( Fraunhofer Institute for Molecular Biology and Applied Ecology (Fraunhofer IME), 57392 Schmallenberg, Germany. heinz.ruedel@ime.fraunhofer.de)
Abstract	BACKGROUND AND AIMS: Hexabromocyclododecane (HBCD) is a brominated flame retardant used mainly in polystyrene foam as well as in textile applications. In recent years, measures were taken to reduce HBCD emissions during its production and use. To evaluate the efficacy of these measures, a monitoring project was initiated with fish as bioaccumulation indicators. METHODS: Since 2007 bream was sampled annually at several European freshwater sites applying standardized methods. Muscle samples were analyzed by a validated liquid chromatography-tandem mass spectrometry (LC-MS/MS) method which allows the quantification of -, ß-, and Î³-diastereomers of HBCD. DISCUSSION: In most samples, -HBCD was predominant. The lowest HBCD levels (11 µg/kg lipid weight (lw), sum of three HBCD diastereomers) were detected in bream sampled in 2009 from Lake Belau which is situated in a rural area of Northern Germany. During the 4-year study period, statistical significant decreases of HBCD concentrations were detected in bream from the rivers Rhone (France; -85%, level 2010, 205 µg/kg lw) and Western Scheldt (the Netherlands; -60%, level 2010, 36 µg/kg lw). High HBCD concentrations (9,480-14,500 µg/kg lw) without a clear time trend were observed in bream from the river Tees (UK). These high levels are in line with published data for fish from contaminated regions. CONCLUSIONS: Overall, the results indicate that environmental burdens of HBCD are decreasing at those locations where point sources and more diffuse emissions are expected.
ISSN	09441344
Issue Number	3
Volume Number	19
e-ISSN	16147499
Journal	Environmental Science and Pollution Research
Language	English
Publisher	Springer
Publisher Date	2012-03-01
Publisher Place	Germany
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Cyprinidae Flatfishes Fresh Water Hydrocarbons, Brominated Analysis Muscles Chemistry Seawater Water Pollutants, Chemical Animals Biometry Chromatography, High Pressure Liquid Growth & Development Environmental Monitoring Methods Europe Flame Retardants Hydrophobic And Hydrophilic Interactions Lipids Spectrometry, Mass, Electrospray Ionization Stereoisomerism Tandem Mass Spectrometry Time Factors Comparative Study Journal Article Research Support, Non-u.s. Gov't Validation Studies Discipline Environmental Science Discipline Environmental Chemistry
Content Type	Text
Resource Type	Article
Subject	Environmental Chemistry Health, Toxicology and Mutagenesis Pollution Medicine

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