NDLI: Effects of operating conditions on trihalomethanes formation and speciation during chloramination in reclaimed water

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Effects of operating conditions on trihalomethanes formation and speciation during chloramination in reclaimed water

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Li, Qian Ma, Defang Li, Ruihua Gao, Baoyu Sun, Shenglei Wang, Fang Yue, Qinyan Wang, Yan
Spatial Coverage	China
Description	Country affiliation: China Author Affiliation: Wang F ( Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Ji' nan, 250100, China.); Gao B ( Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Ji' nan, 250100, China. baoyugao_sdu@aliyun.com.); Ma D ( Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Ji' nan, 250100, China.); Li R ( Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Ji' nan, 250100, China.); Sun S ( Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Ji' nan, 250100, China.); Yue Q ( Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Ji' nan, 250100, China.); Wang Y ( Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Ji' nan, 250100, China.); Li Q ( Shandong Key Laboratory of Water Pollution Control and Resource Reuse, School of Environmental Science and Engineering, Shandong University, Ji' nan, 250100, China.)
Abstract	In this study, a hybrid powdered activated carbon-membrane bioreactor (PAC-MBR) system was used to treat municipal wastewater in northern China intended for recycle. In order to control microbiological hazards in PAC-MBR effluent, chloramine was chosen as the disinfectant which could reduce the disinfection by-product yields. Effects of reaction time, chloramines dose, pH value, and bromide ion concentration on trihalomethanes (THMs) formation and speciation during chloramination of the reclaimed effluent were investigated. Study results indicated that the yield of total THMs (TTHM) increased at higher reaction time and chloramines dose. The trend of growth showed that slow reacting precursors were the main components of dissolved organic matter (DOM) in PAC-MBR effluent. THMs formation potential of PAC-MBR effluent achieved the maximum at chloramines dosage of 20 mg/L. Meanwhile, THMs formation was enhanced evidently under alkaline conditions. The yields of THMs species were in following order: $CHCl_{3}$ > $CHBrCl_{2}$ > $CHBr_{2}Cl$ > $CHBr_{3},$ although in different reaction time, chloramines dose, and pH value. Furthermore, the formation of Br-THMs was promoted by the increasing concentration of bromide ion.
ISSN	09441344
Issue Number	2
Volume Number	23
e-ISSN	16147499
Journal	Environmental Science and Pollution Research
Language	English
Publisher	Springer
Publisher Date	2016-01-01
Publisher Place	Germany
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Chloramines Chemistry Trihalomethanes Analysis Waste Water Water Purification Bioreactors Charcoal China Disinfectants Disinfection Methods Halogenation Water Water Pollutants, Chemical Journal Article Research Support, Non-u.s. Gov't Discipline Environmental Science Discipline Environmental Chemistry
Content Type	Text
Resource Type	Article
Subject	Environmental Chemistry Health, Toxicology and Mutagenesis Pollution Medicine

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