NDLI: From cage-in-cage MOF to N-doped and Co-nanoparticle-embedded carbon for oxygen reduction reaction

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From cage-in-cage MOF to N-doped and Co-nanoparticle-embedded carbon for oxygen reduction reaction

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From cage-in-cage MOF to N-doped and Co-nanoparticle-embedded carbon for oxygen reduction reaction

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Lin, Qipu Kong, Aiguo Bu, Xianhui Mao, Chengyu Wei, Xiao Feng, Pingyun
Description	Author Affiliation: Kong A ( Department of Chemistry, University of California, Riverside, California 92521, USA. pingyun.feng@ucr.edu.)
Abstract	By one-step pyrolysis of a unique “cage-in-cage” cobalt metal–organic framework, nitrogen-doped carbon cubes embedded with numerous metallic Co nanoparticles were obtained. A considerable amount of Co particles was encapsulated in thin carbon shells and formed the core–shell-like Co@C structure. With about 60 wt% Co particles in the prepared sample, the nanocomposites of Co nanoparticles and nitrogen-doped carbon show electrocatalytic activity for the oxygen reduction reaction (ORR) with an efficiency comparable to the commercial Pt/C catalyst, but with better durability and methanol-tolerance performance. The metallic Co nanoparticles were found to play an important role in enhancing the ORR activity of the nanocomposites. This simple one-step pyrolysis method provides a novel synthetic route for the synthesis of core–shell-like Co@C nano-composites. The synthesized material represents a highly active non-precious metal catalyst for ORR.
ISSN	14779226
Issue Number	15
Journal	Dalton Trans.
Volume Number	44
e-ISSN	13645447
Language	English
Publisher	Royal Society of Chemistry
Publisher Date	2015-04-21
Publisher Place	Great Britain (UK)
Access Restriction	Subscribed
Subject Keyword	Chemistry
Content Type	Text
Resource Type	Article
Subject	Inorganic Chemistry

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