NDLI: Synthesis and Morphogenesis of Organic and Inorganic Polymers by Means of Biominerals and Biomimetic Materials

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Alkaline Earth Metal Ion Induced Coil–Helix–Coil Transition of Lysine–Coumarin–Azacrown Hybrid Foldamers with OFF–OFF–ON Fluorescence Switching

Synthesis of 2′-Deoxy-1′-homo-N-nucleosides with Anti-Influenza Activity by Catalytic Methyltrioxorhenium $(MTO)/H_{2}O_{2}$ Oxyfunctionalization

Highly Sensitive and Selective Spectroscopic Detection of Mercury(II) in Water by Using Pyridylporphyrin–DNA Conjugates

Fine-Tuning the Reactivity and Stability by Systematic Ligand Variations in $CpCo^{I}$ Complexes as Catalysts for [2+2+2] Cycloaddition Reactions

$Ag/AgBr/Co–Ni–NO_{3}$ Layered Double Hydroxide Nanocomposites with Highly Adsorptive and Photocatalytic Properties

Asymmetric Hydrogenation Using Rhodium Complexes Generated from Mixtures of Monodentate Neutral and Anionic Phosphorus Ligands

Hierarchical Self-Assembly of a Biomimetic Light-Harvesting Antenna Based on DNA G-Quadruplexes

Rhodium-Catalyzed [2+2+2] Cycloaddition of Oximes and Diynes To Give Pyridines

Synthesis, Structure, and Single-Molecule Magnetic Properties of Rare-Earth Sandwich Complexes with Mixed Phthalocyanine and Schiff Base Ligands

An Unsymmetrically π-Extended Porphyrin-Based Single-Crystal Field-Effect Transistor and Its Anisotropic Carrier-Transport Behavior

A Modular Synthesis of Teraryl-Based α-Helix Mimetics, Part 2: Synthesis of 5-Pyridine Boronic Acid Pinacol Ester Building Blocks with Amino Acid Side Chains in 3-Position

Microenvironment Effects in Electrocatalysis: Ionic-Liquid-Like Coating on Carbon Nanotubes Enhances the Pd-Electrocatalytic Alcohol Oxidation

TetrathiafulvaleneBenzothiadiazoles as Redox-Tunable Donor–Acceptor Systems: Synthesis and Photophysical Study

A Modular Synthesis of Teraryl-Based α-Helix Mimetics, Part 1: Synthesis of Core Fragments with Two Electronically Differentiated Leaving Groups

Palladium-Catalyzed Intermolecular Desulfinylative Cross-Coupling of Heteroaromatic Sulfinates

Anodic-Stripping Voltammetric Immunoassay for Ultrasensitive Detection of Low-Abundance Proteins Using Quantum Dot Aggregated Hollow Microspheres

Design and Synthesis of a New Family of Fluorinated Liquid Crystals

Isomerization Energy Decomposition Analysis for Highly Ionic Systems: Case Study of Starlike $E_{5}Li_{7}^{+}$ Clusters

Collective Total Synthesis of Englerin A and B, Orientalol E and F, and Oxyphyllol: Application of the Organocatalytic [4+3] Cycloaddition Reaction

Inner Workings of a Cinchona Alkaloid Catalyzed Oxa-Michael Cyclization: Evidence for a Concerted Hydrogen-Bond-Network $Mechanism^{†}$

Syntheses and Characterization of New Vinyl-Borylene Complexes by the Hydroboration of Alkynes with $[(μ_{3}-BH)(Cp*RuCO)_{2}(μ-CO)Fe(CO)_{3}]^{†}$

Facile Electrochemical Oxidation of Polyaromatic Hydrocarbons to Surface-Confined Redox-Active Quinone Species on a Multiwalled Carbon Nanotube Surface

Generation of Molecular Complexity from Cyclooctatetraene: Preparation of Optically Active Protected Aminocycloheptitols and Bicyclo[4.4.1]undecatriene

An Efficient Method for Sterically Demanding Suzuki–Miyaura Coupling Reactions

Phospholipid–Detergent Conjugates as Novel Tools for siRNA Delivery

$[(η^{6}-Praziquantel)Cr(CO)_{3}]$ Derivatives with Remarkable In Vitro Anti-schistosomal Activity

Diastereoselective Access to Polyoxygenated Polycyclic Spirolactones through a Rhodium-Catalyzed [3+2] Cycloaddition Reaction: Experimental and Theoretical Studies

$C_{5}Li_{7}^{+}$ and $O_{2}Li_{5}^{+}$ as Noble-Gas-Trapping Agents

The Hydride-Ion Affinity of Borenium Cations and Their Propensity to Activate $H_{2}$ in Frustrated Lewis Pairs

A New Modular Phosphite-Pyridine Ligand Library for Asymmetric Pd-Catalyzed Allylic Substitution Reactions: A Study of the Key Pd-π-Allyl Intermediates

S-Alkylation of Soft Scorpionates

Gold(I) and Silver(I) Complexes of Diphosphacyclobutadiene Cobaltate Sandwich Anions

Cross-Linked Helically Chiral Poly-(γ-benzyl-L-glutamate) as Enantiodiscriminating Alignment Medium

Synthesis and Thermoreversible Gelation Properties of Main-Chain Poly(pyridine-2,6-dicarboxamide-triazole)s

Ionic-Liquid-Assisted Synthesis of Uniform Fluorinated B/C-Codoped $TiO_{2}$ Nanocrystals and Their Enhanced Visible-Light Photocatalytic Activity

Electrochemical Deposition of Mesoporous Pt–Au Alloy Films in Aqueous Surfactant Solutions: Towards a Highly Sensitive Amperometric Glucose Sensor

Cascade Syntheses Routes to the Centrocountins

Nitrogen-Doped Carbon Dots: A Facile and General Preparation Method, Photoluminescence Investigation, and Imaging Applications

Synthesis and Morphogenesis of Organic and Inorganic Polymers by Means of Biominerals and Biomimetic Materials

Stereoselective Multiple Bond-Forming Transformations (MBFTs): The Power of 1,2- and 1,3-Dicarbonyl Compounds

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Synthesis and Morphogenesis of Organic and Inorganic Polymers by Means of Biominerals and Biomimetic Materials

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Munekawa, Yurika Oaki, Yuya Imai, Hiroaki Kijima, Misako
Description	Author Affiliation: Kijima M ( Department of Applied Chemistry, Faculty of Science and Technology, Keio University, 3-14-1 Hiyoshi, Kohoku-ku, Yokohama 223-8522, Japan.)
Abstract	We have studied the simultaneous synthesis and morphogenesis of polymer materials with hierarchical structures from nanoscopic to macroscopic scales. The morphologies of the original materials can be replicated to the polymer materials. In general, it is not easy to achieve the simultaneous synthesis and morphogenesis of polymer material even using host materials. In the present work, four biominerals and three biomimetic mesocrystal structures are used as the host materials or templates and polypyrrole, poly(3-hexylthiopehene), and silica were used as the precursors for the simultaneous syntheses and morphogenesis of polymer materials. The host materials with the hierarchical structure possess the nanospace for the incorporation of the monomers. After the incorporation of the monomers, the polymerization reaction proceeds in the nanospace with addition of the initiator agents. Then, the dissolution of the host materials leads to the formation and morphogenesis of the polymer materials. The scheme of the replication can be classified into the three types based on the structures of the host materials (types I–III). The type I template facilitates the hierarchical replication of the whole host material, type II mediates the hierarchical surface replication, and type III induces the formation of the two-dimensional nanosheets. Based on these results, the approach for the coupled synthesis and morphogenesis can be applied to a variety of combinations of the templates and polymer materials.
ISSN	09476539
e-ISSN	15213765
Journal	Chemistry - A European Journal
Issue Number	7
Volume Number	19
Language	English
Publisher	Wiley-VCH;ChemPubSoc Europe
Publisher Date	2013-02-11
Publisher Place	Germany
Access Restriction	Open
Subject Keyword	Biomimetic Materials Chemistry Chemical Synthesis Polymers Pyrroles Chemistry, Inorganic Morphogenesis Organic Chemistry Phenomena Polymerization Research Support, Non-U.S. Gov't
Content Type	Text
Resource Type	Article
Subject	Organic Chemistry Catalysis

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