NDLI: Supracolloidal Architectures Self-Assembled in Microdroplets

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Supracolloidal Architectures Self-Assembled in Microdroplets

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Supracolloidal Architectures Self-Assembled in Microdroplets

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Parker, Richard M. Abell, Chris Wu, Yuchao Xu, Xuejiao Scherman, Oren A. Liu, Xin Yu, Ziyi Lan, Yang Tian, Feng
Description	Author Affiliation: Xu X ( Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2â 1EW (UK).); Tian F ( Melville Laboratory for Polymer Synthesis, Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2â 1EW (UK).); Liu X ( Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2â 1EW (UK).); Parker RM ( Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2â 1EW (UK).); Lan Y ( Melville Laboratory for Polymer Synthesis, Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2â 1EW (UK).); Wu Y ( Melville Laboratory for Polymer Synthesis, Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2â 1EW (UK).); Yu Z ( Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2â 1EW (UK).); Scherman OA ( Melville Laboratory for Polymer Synthesis, Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2â 1EW (UK). oas23@cam.ac.uk.); Abell C ( Department of Chemistry, University of Cambridge, Lensfield Road, Cambridge CB2â 1EW (UK). ca26@cam.ac.uk.)
Abstract	We demonstrate a novel method for the formation of a library of structured colloidal assemblies by exploiting the supramolecular heteroternary host–guest interaction between cucurbit[8]uril (CB[8]) and methyl viologen- and naphthalene-functionalised particles. The approach is dependent upon compartmentalisation in microdroplets generated by a microfluidic platform. Though the distribution of colloidal particles encapsulated within each microdroplet followed a Poisson distribution, tuning the concentration of the initial colloidal particle suspensions provided some level of control over the structure of the formed colloidal assemblies. This ability to direct the assembly of complementarily-functionalised colloids through a supramolecular interaction, without the need for complex modification of the colloidal surface or external stimuli, presents an exciting new approach towards the design of structured colloidal materials with the potential to produce many challenging structures.
ISSN	09476539
e-ISSN	15213765
Journal	Chemistry - A European Journal
Issue Number	44
Volume Number	21
Language	English
Publisher	Wiley-VCH;ChemPubSoc Europe
Publisher Date	2015-10-26
Publisher Place	Germany
Access Restriction	Open
Subject Keyword	Chemistry
Content Type	Text
Resource Type	Article
Subject	Organic Chemistry Catalysis

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