NDLI: Photochemical production of carbonyl sulfide, carbon disulfide and dimethyl sulfide in a lake water.

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Photochemical production of carbonyl sulfide, carbon disulfide and dimethyl sulfide in a lake water.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Du, Qianqian Mu, Yujing Zhang, Chenglong Liu, Junfeng Zhang, Yuanyuan Liu, Chengtang
Spatial Coverage	Beijing
Description	Author Affiliation: Du Q ( Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China); Mu Y ( Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China); Zhang C ( Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China); Liu J ( Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China); Zhang Y ( Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China); Liu C ( Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China)
Abstract	Photochemical production of carbonyl sulfide (COS), carbon disulfide (CS ) and dimethyl sulfide (DMS) was intensively studied in the water from the Aohai Lake of Beijing city. The lake water was found to be highly supersaturated with COS, CS and DMS, with their initial concentrations of 0.91±0.073nmol/L, 0.55±0.071nmol/L and 0.37±0.062nmol/L, respectively. The evident photochemical production of COS and CS in the lake water under irradiation of 365nm and 302nm indicated that photochemical production of them might be the reason for their supersaturation. The similar dependence of wavelength and oxygen for photochemical production of COS, CS and DMS implied that they might be from the same precursors. The water cage effect was found to favor COS production but inhibit CS and DMS formation, indicating that COS photochemical production was mainly from direct degradation of the precursors and the formation of CS and DMS needed intermediates via combination of carbon-centered radicals and sulfur-centered radicals. The above assumptions were further confirmed by simulation experiments with addition of carbonyls and amino acids (cysteine and methionine), and the photochemical formation mechanisms for COS, CS and DMS in water were derived from the investigations.
File Format	HTM / HTML
ISSN	10010742
Volume Number	51
Journal	Journal of Environmental Sciences
Language	English
Publisher	Elsevier
Publisher Date	2017-01-01
Publisher Place	Netherlands
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Discipline Environmental Health Carbon Disulfide Chemistry Lakes Models, Chemical Photochemical Processes Sulfides Sulfur Oxides Water Pollutants, Chemical Beijing Journal Article
Content Type	Text
Resource Type	Article
Subject	Environmental Chemistry Medicine Environmental Engineering

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