NDLI: High-Surface-Area Carbon Molecular Sieves for Selective $CO

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High-Surface-Area Carbon Molecular Sieves for Selective $CO_{2}$ Adsorption

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Wahby, Anass Ramos-Fernández, José M. Martínez-Escandell, Manuel Sepúlveda-Escribano, Antonio Silvestre-Albero, Joaquín Rodríguez-Reinoso, Francisco
Description	Country affiliation: Spain Author Affiliation: Wahby A ( Departamento de Química Inorgánica-Instituto Universitario de Materiales, Universidad de Alicante, Spain.)
Abstract	A series of carbon molecular sieves (CMSs) has been prepared, either as powders or monoliths, from petroleum pitch using potassium hydroxide as the activating agent. The CMS monoliths are prepared without the use of a binder based on the self-sintering ability of the mesophase pitch. Characterization results show that these CMSs combine a large apparent surface area (up to $ca. 3100 m^{2} g^{−1})$ together with a well-developed narrow microporosity $(V_{n}$ up to $ca. 1.4 cm^{3} g^{−1}).$ The materials exhibit high adsorption capacities for $CO_{2}$ at 1 bar and 273 K (up to $ca. 380 mg CO_{2} g sorbent^{−1}).$ To our knowledge, this is the best result obtained for $CO_{2}$ adsorption using carbon-based materials. Furthermore, although the $CO_{2}$ adsorption capacity for activated carbons has usually been considered lower than that of zeolites, the reported values exceed the total amount adsorbed on traditional 13X and 5A zeolites (ca. 230 mg and $180 mg CO_{2} g sorbent^{−1},$ respectively), under identical experimental conditions. Additionally, the narrow pore openings found in the CMS samples (ca. 0.4 nm) allows for the selective adsorption of $CO_{2}$ from molecules of similar dimensions (e.g., $CH_{4}$ and $N_{2}).$
File Format	HTM / HTML
ISSN	18645631
Issue Number	8
Volume Number	3
e-ISSN	1864564X
Journal	ChemSusChem
Language	English
Publisher	Wiley-VCH
Publisher Date	2010-08-23
Publisher Place	Germany
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Methane Research Support, Non-u.s. Gov't Temperature Discipline Sustainable Chemistry Isolation & Purification Carbon Sequestration Nitrogen Carbon Dioxide Journal Article Chemistry Adsorption Surface Properties Kinetics Porosity
Content Type	Text
Resource Type	Article
Subject	Energy Environmental Chemistry Materials Science Chemical Engineering

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