NDLI: Selective aerobic oxidation of HMF to 2,5-diformylfuran on covalent triazine frameworks-supported Ru catalysts.

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Selective aerobic oxidation of HMF to 2,5-diformylfuran on covalent triazine frameworks-supported Ru catalysts.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Artz, Jens Mallmann, Sabrina Palkovits, Regina
Description	Author Affiliation: Artz J ( Chair of Heterogeneous Catalysis & Chemical Technology, Institut für Technische und Makromolekulare Chemie, RWTH Aachen University, Worringerweg 1, 52074 Aachen (Germany).)
Abstract	The selective aerobic oxidation of 5-hydroxymethylfurfural (HMF) to 2,5-diformylfuran has been performed under mild conditions at 80 °C and 20âbar of synthetic air in methyl t-butyl ether. Ru clusters supported on covalent triazine frameworks (CTFs) allowed excellent selectivity and superior catalytic activity compared to other support materials such as activated carbon, Î³-Al2 O3 , hydrotalcite, or MgO. CTFs with varying pore size, specific surface area, and N content could be prepared from different monomers. The structural properties of the CTF materials influence the catalytic activity of Ru/CTF significantly in the aerobic oxidation of HMF, which emphasizes the superior activity of mesoporous CTFs. Recycling of the catalysts is challenging, but promising methods to maintain high catalytic activity were developed that facilitate only minor deactivation in five consecutive recycling experiments.
File Format	HTM / HTML
ISSN	18645631
Issue Number	4
Volume Number	8
e-ISSN	1864564X
Journal	ChemSusChem
Language	English
Publisher	Wiley-VCH
Publisher Date	2015-02-01
Publisher Place	Germany
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Triazines Research Support, Non-u.s. Gov't Chemistry Ruthenium Oxidation-reduction Discipline Sustainable Chemistry Furans Furaldehyde Catalysis Analogs & Derivatives Journal Article Metal Nanoparticles
Content Type	Text
Resource Type	Article
Subject	Energy Environmental Chemistry Materials Science Chemical Engineering

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