NDLI: Carbon Nanotubes as Support in the Platinum-Catalyzed Hydrolytic Dehydrogenation of Ammonia Borane.

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Carbon Nanotubes as Support in the Platinum-Catalyzed Hydrolytic Dehydrogenation of Ammonia Borane.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Chen, Wenyao Duan, Xuezhi Qian, Gang Chen, De Zhou, Xinggui
Description	Author Affiliation: Chen W ( State Key Laboratory of Chemical Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai 200237(PR China).); Duan X ( State Key Laboratory of Chemical Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai 200237(PR China). xzduan@ecust.edu.cn.); Qian G ( Department of Chemical Engineering, Norwegian University of Science and Technology, 7491 Trondheim (Norway). xzduan@ecust.edu.cn.); Chen D ( State Key Laboratory of Chemical Engineering, East China University of Science and Technology, 130 Meilong Road, Shanghai 200237(PR China).); Zhou X ( Department of Chemical Engineering, Norwegian University of Science and Technology, 7491 Trondheim (Norway). chen@nt.ntnu.no.)
Abstract	We report remarkable support effects for carbon nanotubes (CNTs) in the Pt/CNT-catalyzed hydrolytic dehydrogenation of ammonia borane. The origin of the support-dependent activity and durability is elucidated by combining the catalytic and durability testing with characterization by a range of spectroscopy and high-angle annular dark-field scanning transmission electron microscopy techniques and ICP analysis. The effects mainly arise from different electronic properties and different abilities for the adsorption of boron-containing species on platinum surfaces and changes in size and shape of the platinum particles during the reaction. Defect-rich CNTs in particular are a promising support material, as it not only enhances the platinum binding energy, leading to the highest hydrogen generation rate, but also inhibits the adsorption of boron-containing species and stabilizes the platinum nanoparticles to resist the agglomeration during the reaction, leading to the highest durability. The insights revealed herein may pave the way for the rational design of highly active and durable metal/carbon catalysts for the hydrolytic dehydrogenation of ammonia borane.
File Format	HTM / HTML
ISSN	18645631
Issue Number	17
Volume Number	8
e-ISSN	1864564X
Journal	ChemSusChem
Language	English
Publisher	Wiley-VCH
Publisher Date	2015-09-07
Publisher Place	Germany
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Hydrolysis Ammonia Research Support, Non-u.s. Gov't Chemistry Nanotubes, Carbon Hydrogen Platinum Discipline Sustainable Chemistry Boranes Catalysis Journal Article
Content Type	Text
Resource Type	Article
Subject	Energy Environmental Chemistry Materials Science Chemical Engineering

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Carbon Nanotubes as Support in the Platinum-Catalyzed Hydrolytic Dehydrogenation of Ammonia Borane. : Corrigendum

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Carbon Nanotubes as Support in the Platinum-Catalyzed Hydrolytic Dehydrogenation of Ammonia Borane.

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