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Selective gas-phase oxidation of ethanol by molecular oxygen over oxide and gold-containing catalysts

Content Provider	Springer Nature Link
Author	Koltunov, K. Yu. Sobolev, V. I.
Copyright Year	2012
Abstract	The rapid increase in the production rates of bioalcohols (in particular bioethanol) gives grounds for regarding them as a promising renewable chemical raw material for obtaining a number of useful organic synthesis products. In order to develop new green technologies for processing ethanol into value-added products, a systematic study of selective conversion of ethanol under conditions of oxidation by molecular oxygen in the flow gas-phase mode over such catalysts as V$_{2}$O$_{5}$-TiO$_{2}$, mixed oxides V-Mo-Te, V-Mo-Nb and V-Mo-Te-Nb, and gold supported on oxide supports is performed. The catalytic activity is determined under conditions of temperature-programmed reaction under atmospheric pressure using a gas mixture (composition, mol %: EtOH, 2; O$_{2}$, 18; He, 80) at a hourly space velocity of the mixture of 3600 h$^{−1}$ over 0.25–0.5 mm catalyst fraction. The possibility of the efficient conversion of ethanol to products of partial oxidation and accompanying conversions (acetaldehyde, 90–99% yield; acetic acid, 92-98% yield; productive capacity >3 g g-cat$^{−1}$ h$^{−1}$) and acetic acid-ethyl acetate mixtures (1: 1 ratio, total yield >90%) in a number of cases is demonstrated.
Starting Page	247
Ending Page	252
Page Count	6
File Format	PDF
ISSN	20700504
Journal	Catalysis in Industry
Volume Number	4
Issue Number	4
e-ISSN	20700555
Language	English
Publisher	SP MAIK Nauka/Interperiodica
Publisher Date	2012-12-16
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	selective gas-phase oxidation ethanol acetaldehyde acetic acid heterogeneous catalysis Catalysis
Content Type	Text
Resource Type	Article
Subject	Catalysis

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Selective gas-phase oxidation of ethanol by molecular oxygen over oxide and gold-containing catalysts

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