NDLI: Visible-light-induced oxidative removal of nitrogen oxides in air by metal chloride-modified titanium (IV) oxide nanoparticles

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Visible-light-induced oxidative removal of nitrogen oxides in air by metal chloride-modified titanium (IV) oxide nanoparticles

Content Provider	Springer Nature Link
Author	Kominami, Hiroshi Sumida, Katutoshi Yamamoto, Kazuto Kondo, buaki Hashimoto, Keiji Kera, Yoshiya
Copyright Year	2008
Abstract	Various metal chloride-modified titanium(IV) oxide (TiO$_{2}$) (MCMT) samples were prepared by loading metal chloride on commercial TiO$_{2}$ nanoparticles (Ishihara ST-01) having a large specific surface area and used for photoinduced oxidative removal of nitrogen oxides (NO$_{ x }$) in air under irradiation of visible light and/or ultraviolet (UV) light. The NO$_{ x }$ removal activity of MCMT samples under photoirradiation from a blue fluorescent lamp (BFL) with a UV cut filter decreased in the following order: RhCl$_{3}$/ST-01>H$_{2}$PtCl$_{6}$/ST-01>RuCl$_{3}$/ST-01>ST-01>IrCl$_{4}$/ST-01>HAuCl$_{4}$/ST-01, indicating that RhCl$_{3}$. H$_{2}$PtCl$_{6}$ and RuCl$_{3}$ fixed on TiO$_{2}$ effectively worked as photosensitizers for NO$_{ x }$ removal. NO$_{ x }$ was almost quantitatively fixed as nitrate on RhCl$_{3}$/ST-01 photoirradiated with BFL or blue light-emitting diodes. Under irradiation of both visible light and UV light from a white fluorescent lamp, RhCl$_{3}$/ST-01 exhibited a higher level of removal of NO$_{ x }$ and a much lower level of release of nitrogen dioxide than did bare ST-01, indicating that RhCl$_{3}$/ST-01 effectively utilized both visible light and UV light and that two types of reaction (photosensitization by fixed RhCl$_{3}$ and photocatalysis by TiO$_{2}$) occurred over RhCl$_{3}$/ST-01.
Starting Page	587
Ending Page	601
Page Count	15
File Format	PDF
ISSN	09226168
Journal	Research on Chemical Intermediates
Volume Number	34
Issue Number	5-7
e-ISSN	15685675
Language	English
Publisher	Springer Netherlands
Publisher Date	2008-01-01
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Metal chlorides titanium(IV) oxide nitrogen oxides visible light photosensitization photocatalysis Catalysis Physical Chemistry Inorganic Chemistry
Content Type	Text
Resource Type	Article
Subject	Chemistry

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