NDLI: An Integrated Approach to Understanding the Mass Transfer and Reaction Processes in a Pulsed High-Voltage Discharge Reactor

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An Integrated Approach to Understanding the Mass Transfer and Reaction Processes in a Pulsed High-Voltage Discharge Reactor

Content Provider	Springer Nature Link
Author	Zeng, Mengdan Zhao, Kang Lu, Yang Ouyang, Yongjian Liu, Deqi Wang, Mei Ma, Yimei
Copyright Year	2015
Abstract	The effect of pulsed high-voltage discharge on mass transfer and reaction processes in a needle-plate reactor was studied. Bubble size distributions and characteristic parameters were determined by photography, implying that inlet air bubbles could be broken into smaller ones effectively by discharge. The mass transfer parameters including specific interfacial area (a), volumetric mass transfer coefficient (k $_{L}$ a), and liquid-side mass transfer coefficient (k $_{L}$) were obtained by Danckwerts-plot, reflecting the mass transfer processes. In addition, 4-chlorophenol (4-CP) decomposition was determined under the same experimental conditions. The results showed that the conclusions of 4-CP removal were coincided with the statistical results of bubble images, illustrating that higher peak voltage, pulsed frequency and appropriate air flow rate are beneficial to mass transfer and reaction. However, there was a slight difference between 4-CP removal and mass transfer parameters at higher air flow rate. Therefore, it is more reasonable to optimize the operating conditions of a pulsed high-voltage discharge reactor via combining image acquisition and mass transfer parameters with the results of pollutant degradation.
Starting Page	721
Ending Page	738
Page Count	18
File Format	PDF
ISSN	02724324
Journal	Plasma Chemistry and Plasma Processing
Volume Number	35
Issue Number	4
e-ISSN	15728986
Language	English
Publisher	Springer US
Publisher Date	2015-03-26
Publisher Place	New York
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Pulsed high-voltage discharge Plasma Bubble size distribution Gas–liquid mass transfer process 4-chlorophenol decomposition Inorganic Chemistry Mechanics Characterization and Evaluation of Materials Mechanical Engineering
Content Type	Text
Resource Type	Article
Subject	Chemistry Surfaces, Coatings and Films Condensed Matter Physics Chemical Engineering

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