NDLI: Ac Conductivity and Transport Properties of [N(C$_{3}$H$_{7}$)$_{4}$]$_{2}$Zn$_{2}$Cl$

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Ac Conductivity and Transport Properties of [N(C$_{3}$H$_{7}$)$_{4}$]$_{2}$Zn$_{2}$Cl$_{6}$ Compound

Content Provider	Springer Nature Link
Author	Ben Gzaiel, M. Oueslati, A. Gargouri, M.
Copyright Year	2015
Abstract	The electrical properties and ac conductivity of the bis tetra-propylammonium hexachloro-dizincate have been investigated by means of impedance spectroscopy measurements in the 209 Hz–5 MHz frequency range and 303–403 K temperature interval. The Nyquist plots are fitted to an equivalent circuit modeled by a combination of a parallel bulk resistance and constant phase elements. The experimental results indicate that σ$_{ac}$(ω) is proportional to (ω$^{s}$). It was found that s increases by increasing temperature below the phase transition at 327 ± (5) K (region I) and decrease with increasing temperature above 327 ± (5) (region II). An agreement between the experimental and theoretical results are discussed and suggests that the ac conductivity can be explained by the non overlapping small polaron tunneling model and correlated barrier hopping in region I and II, respectively. Furthermore, the modulus plots can be characterized by full width at half height or in terms of a non-experiential decay function $$\varPhi \left( {\text{t}} \right) = \exp \left( {\frac{{ - {\text{t}}}}{\tau }} \right)^{\beta }$$ .
Starting Page	1577
Ending Page	1594
Page Count	18
File Format	PDF
ISSN	10407278
Journal	Journal of Cluster Science
Volume Number	26
Issue Number	5
e-ISSN	15728862
Language	English
Publisher	Springer US
Publisher Date	2015-02-17
Publisher Place	New York
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Bis tetra-propylammonium hexachloro-dizincate Equivalent circuit Ac conductivity Modulus analysis Catalysis Inorganic Chemistry Physical Chemistry Nanochemistry
Content Type	Text
Resource Type	Article
Subject	Chemistry Biochemistry Condensed Matter Physics Materials Science

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