NDLI: Salicylaldimine difluoroboron complexes containing <i>tert</i>-butyl groups: nontraditional π-gelator and piezofluorochromic compounds

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Salicylaldimine difluoroboron complexes containing tert-butyl groups: nontraditional π-gelator and piezofluorochromic compounds

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Journal of Materials Chemistry C Vol - 3 Issue - 29

Journal of Materials Chemistry C Vol - 3 Issue - 19

Journal of Materials Chemistry C Vol - 3 Issue - 9

Journal of Materials Chemistry C Vol - 3 Issue - 8

Journal of Materials Chemistry C Vol - 3 Issue - 7

Journal of Materials Chemistry C Vol - 3 Issue - 6

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Journal of Materials Chemistry C Vol -1

Salicylaldimine difluoroboron complexes containing tert-butyl groups: nontraditional π-gelator and piezofluorochromic compounds

Content Provider	Royal Society of Chemistry (RSC)
Author	Gong, Peng Yang, Hao Xue, Pengchong Sun, Jiabao Zhang, Zhenqi Sun, Jingbo Lu, Ran
Copyright Year	2015
Abstract	We have synthesized three new salicylaldimine difluoroboron complexes with tert-butyl groups 1B–3B, which are highly emissive in solutions and in solid states. It was found that salicylaldehydehydrazone difluoroboron complex 1B could form organogels in n-hexane and the mixture of petroleum ether/CH2Cl2, and 1D nanoribbons with intense blue emission could be fabricated via the gelation of the nontraditional organogelator 1B directed by balanced π–π interaction. However, the other two salicylaldimine difluoroboron complexes 2B and 3B with a spacer of the benzene ring could not form a gel due to the strong π–π interaction, but exhibited piezofluorochromic behaviors. The as-prepared crystals of 2B and 3B giving blue-green fluorescence could be transformed into the powders emitting yellow light upon grinding, and the emission could recover when the ground powders were heated. It suggested that the reversible piezofluorochromism originated from the transformation between crystalline and amorphous states. It provided a strategy for designing new nontraditional π-gelators and piezofluorochromic materials via tuning the π–π interaction.
Starting Page	10302
Ending Page	10308
Page Count	7
File Format	HTM / HTML PDF
ISSN	20507526
Volume Number	3
Issue Number	39
Journal	Journal of Materials Chemistry C
DOI	10.1039/c5tc02484f
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Butyl group Organogels Hexane Petroleum ether Benzene Fluorescence
Content Type	Text
Resource Type	Article
Subject	Chemistry Materials Chemistry

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Salicylaldimine difluoroboron complexes containing tert-butyl groups: nontraditional π-gelator and piezofluorochromic compounds

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