NDLI: Use of ion-selective polymer membranes for an aqueous electrolyte rechargeable Li-ion

Content Provider	Royal Society of Chemistry (RSC)
Author	Morcrette, Mathieu Tarascon, Jean-Marie Demir-Cakan, Rezan
Copyright Year	2015
Abstract	Aqueous electrolyte Li-ion–polysulphide batteries offer great promise due to the use of low-cost and abundant raw materials. Following up on our previous studies in which we explored a totally new practical battery chemistry coupling a well-known cathode material in Li-ion batteries (i.e. LiMn2O4) with a dissolved polysulphide anode, herein we aim to further develop the system by replacing the ceramic membrane with an ion-selective polymer membrane, allowing cost-effective and higher energy density options. After tuning the osmotic movements inside the membrane, dissolved polysulphide leakage from one compartment to another is successfully eliminated. With the additional use of porous silica serving as an absorbent for sulphur-based gaseous products, a 1.5 V average voltage together with a stable cycling profile over 200 cycles at high current density regimes are easily achieved.
Starting Page	2869
Ending Page	2875
Page Count	7
File Format	HTM / HTML PDF
ISSN	20507488
Volume Number	3
Issue Number	6
Journal	Journal of Materials Chemistry A
DOI	10.1039/c4ta05756b
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Electrolyte Chemistry Cathode Anode Ceramic membrane Polymer Energy density Silicon dioxide Electric current
Content Type	Text
Resource Type	Article
Subject	Chemistry Renewable Energy, Sustainability and the Environment Materials Science

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