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Preparation and catalytic behavior of biomorphic calcium oxide/carbon solid base materials

Content Provider	Royal Society of Chemistry (RSC)
Author	Wang, Lan Chun, Yuan Li, Ting Xu, Qinhua Di, Changmiao
Copyright Year	2015
Abstract	Using plant materials as templates is a convenient and low-cost route to prepare solid base catalysts with high specific surface area. In this study, a series of biomorphic calcium oxide/carbon catalysts have been prepared via an in situ transformation technique using rice grains as a template and carbon precursor. The resulting CaO/carbon materials are spindly shaped catalysts and show a high specific surface area and strong basicity. In the methylation of cyclopentadiene, these CaO/carbon materials exhibit a higher catalytic performance than MgO/carbon materials and CaO prepared by directly calcining the CaO precursor. Moreover, the regeneration of deactivated catalyst is studied, and steam or CO2 treatment at high temperature is found to be very effective for this carbon supported catalyst, and can even promote the catalytic activity. A possible mechanism for the deactivation and regeneration of the CaO/carbon materials has been proposed.
Starting Page	5185
Ending Page	5195
Page Count	11
File Format	HTM / HTML PDF
ISSN	20444753
Volume Number	5
Issue Number	12
Journal	Catalysis Science & Technology
DOI	10.1039/c5cy01028d
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Calcium oxide Cyclopentadiene Solid Base Specific surface area Calcination Methylation Carbon Rice Catalyst support
Content Type	Text
Resource Type	Article
Subject	Catalysis

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