NDLI: Significant roles of mesostructure and basic modifier for ordered mesoporous Ni/CaO–Al2O3 catalyst towards CO2 reforming of CH4

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Catalysis Science & Technology Vol - 4 Issue - 5

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Catalysis Science & Technology Vol - 4 Issue - 3

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Significant roles of mesostructure and basic modifier for ordered mesoporous Ni/CaO–Al₂O₃ catalyst towards CO₂ reforming of CH₄

Content Provider	Royal Society of Chemistry (RSC)
Author	Xu, Leilei Chen, Wei Chou, Lingjun Song, Huanling Miao, Zhichao
Copyright Year	2014
Abstract	An ordered mesoporous CaO–Al2O3 composite oxide had been designed and prepared via improved evaporation induced self-assemble strategy (EISA). The resultant material was utilized as the support of Ni based catalyst for CO2 reforming of CH4. In order to study the roles of the ordered mesopore structure and basic modifier in promoting the catalytic properties toward the CO2 reforming of CH4 reaction, non-mesoporous CaO–Al2O3 without ordered mesostructure and ordered mesoporous Al2O3 without basic modifier were also synthesized, respectively. It was found that both the ordered mesostructure and CaO basic modifier showed significant effects in promoting catalytic activity, stability and suppressing the carbon deposition during their 100 h long term stability tests. Compared with traditional supported catalysts, the confinement effect of the mesoporous catalysts could effectively inhibit the thermal sintering of the Ni particles. Furthermore, the sorts of coke species over the spent catalysts and the mechanism of catalyst deactivation were also carefully investigated. Therefore, the present ordered mesoporous CaO–Al2O3 composite oxide will be a potential carrier for Ni-based catalysts for CO2 reforming of CH4 and even other reactions.
Starting Page	1759
Ending Page	1770
Page Count	12
File Format	HTM / HTML PDF
ISSN	20444753
Volume Number	4
Issue Number	6
Journal	Catalysis Science & Technology
DOI	10.1039/c3cy01037f
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Mesoporous material Sintering Energy Independence and Security Act of 2007 Carbon
Content Type	Text
Resource Type	Article
Subject	Catalysis

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Carbon dioxide reforming of methane over ordered mesoporous NiO–Al₂O₃ composite oxides

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