NDLI: Molecular polypyridine-based metal complexes as catalysts for the reduction of CO<sub>2</sub>

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Chemical Society Reviews Vol -46

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Silica/organosilica cross-linked block copolymer micelles: a versatile theranostic platform

Transition metal-catalyzed cross-coupling reactions using organoindium reagents

Metal-complex chromophores for solar hydrogen generation

Metal complexes with oxygen-functionalized NHC ligands: synthesis and applications

Diamond nanostructures for drug delivery, bioimaging, and biosensing

Molecular polypyridine-based metal complexes as catalysts for the reduction of CO₂

Single lithium-ion conducting solid polymer electrolytes: advances and perspectives

The recent development of efficient Earth-abundant transition-metal nanocatalysts

Macroporous materials: microfluidic fabrication, functionalization and applications

Recent advances in organic thermally activated delayed fluorescence materials

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Chemical Society Reviews Vol - 46 Issue - 2

Chemical Society Reviews Vol - 46 Issue - 1

Chemical Society Reviews Vol -39

Chemical Society Reviews Vol -29

Chemical Society Reviews Vol -19

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Chemical Society Reviews Vol -9

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Chemical Society Reviews Vol -5

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Molecular polypyridine-based metal complexes as catalysts for the reduction of CO₂

Content Provider	Royal Society of Chemistry (RSC)
Author	Elgrishi, Noémie Wang, Xia Fontecave, Marc Chambers, Matthew B.
Copyright Year	2017
Abstract	Polypyridyl transition metal complexes represent one of the more thoroughly studied classes of molecular catalysts towards CO2 reduction to date. Initial reports in the 1980s began with an emphasis on 2nd and 3rd row late transition metals, but more recently the focus has shifted towards earlier metals and base metals. Polypyridyl platforms have proven quite versatile and amenable to studying various parameters that govern product distribution for CO2 reduction. However, open questions remain regarding the key mechanistic steps that govern product selectivity and efficiency. Polypyridyl complexes have also been immobilized through a variety of methods to afford active catalytic materials for CO2 reductions. While still an emerging field, materials incorporating molecular catalysts represent a promising strategy for electrochemical and photoelectrochemical devices capable of CO2 reduction. In general, this class of compounds remains the most promising for the continued development of molecular systems for CO2 reduction and an inspiration for the design of related non-polypyridyl catalysts.
Starting Page	761
Ending Page	796
Page Count	36
File Format	HTM / HTML PDF
ISSN	03060012
Volume Number	46
Issue Number	3
Journal	Chemical Society Reviews
DOI	10.1039/c5cs00391a
Language	English
Publisher	Royal Society of Chemistry
Access Restriction	Open
Subject Keyword	Product selectivity Electrochemistry Photoelectrochemical cell Transition metal
Content Type	Text
Resource Type	Article
Subject	Chemistry

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Molecular polypyridine-based metal complexes as catalysts for the reduction of CO 2

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