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  1. Biosensors
  2. Volume: 4
  3. Issue: 3
  4. Electrochemical Biosensors Based on Ferroceneboronic Acid and Its Derivatives: A Review
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Volume: 8
Volume: 7
Volume: 6
Volume: 5
Volume: 4
Issue: 4
Issue: 3
Microelectrode Arrays and the Use of PEG-Functionalized Diblock Copolymer Coatings
Piezoelectric Biosensors for Organophosphate and Carbamate Pesticides: A Review
Biosensors with Built-In Biomolecular Logic Gates for Practical Applications
Study of Paclitaxel-Treated HeLa Cells by Differential Electrical Impedance Flow Cytometry
Electrochemical Biosensors Based on Ferroceneboronic Acid and Its Derivatives: A Review
Sensing Magnetic Directions in Birds: Radical Pair Processes Involving Cryptochrome
An Inexpensive, Fast and Sensitive Quantitative Lateral Flow Magneto-Immunoassay for Total Prostate Specific Antigen
Magnetic Properties of FeNi-Based Thin Film Materials with Different Additives
Issue: 2
Issue: 1
Volume: 3
Volume: 2
Volume: 1

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Electrochemical Biosensors Based on Ferroceneboronic Acid and Its Derivatives: A Review

Content Provider MDPI
Author Wang, Baozhen Takahashi, Shigehiro Du, Xiaoyan Anzai, Jun-ichi
Abstract We review recent progress in the development of electrochemical biosensors based on ferroceneboronic acid (FcBA) and ferrocene (Fc)-modified boronic acids. These compounds can be used to construct electrochemical biosensors because they consist of a binding site (i.e., a boronic acid moiety) and an electrochemically active part (i.e., an Fc residue). By taking advantage of the unique properties of FcBA and its derivatives, electrochemical sensors sensitive to sugars, glycated hemoglobin (HbA1c), fluoride (F−) ions, and so forth have been widely studied. FcBA-based sugar sensors rely on the selective binding of FcBA to 1,2- or 1,3-diol residues of sugars through the formation of cyclic boronate ester bonds. The redox properties of FcBA-sugar adduct differ from those of free FcBA, which forms the basis of the electrochemical determination of sugars. Thus, non-enzymatic glucose sensors are now being actively studied using FcBA and Fc-modified boronic acids as redox markers. Using a similar principle, HbA1c can be detected by FcBA-based electrochemical systems because it contains hydrocarbon chains on the polypeptide chain. HbA1c sensors are useful for monitoring blood glucose levels over the preceding 8–12 weeks. In addition, FcBA and Fc-modified boronic acids have been used for the detection of F− ions due to the selective binding of boronic acid to F− ions. F−-ion sensors may be useful alternatives to conventional ion-selective electrodes sensitive to F− ion. Furthermore, FcBA derivatives have been studied to construct lectin; steroids; nucleotides; salicylic acid; and bacteria sensors. One of the limitations of FcBA-based sensors comes from the fact that FcBA derivatives are added in sample solutions as reagents. FcBA derivatives should be immobilized on the surface of electrodes for developing reagentless sensors.
File Size 660480
Ending Page 256
Page Count 14
Starting Page 243
File Format PDF
e-ISSN 20796374
DOI 10.3390/bios4030243
Journal Biosensors
Issue Number 3
Volume Number 4
Language English
Publisher Date 2014-07-30
Access Restriction Open
Subject Keyword ferroceneboronic acid ferrocene-modified boronic acid electrochemical sensor glucose sensor HbA1c sensor $F^{−}-ion$ sensor
Content Type Text
Resource Type Article
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