NDLI: Thermoreversibly Cross-Linked EPM Rubber Nanocomposites with Carbon Nanotubes

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Thermoreversibly Cross-Linked EPM Rubber Nanocomposites with Carbon Nanotubes

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Thermoreversibly Cross-Linked EPM Rubber Nanocomposites with Carbon Nanotubes

Content Provider	Directory of Open Access Journals (DOAJ)
Author	Andrea Pucci Lorenzo Massimo Polgar Francesco Criscitiello Machiel van Essen Rodrigo Araya-Hermosilla Nicola Migliore Mattia Lenti Patrizio Raffa Francesco Picchioni
Abstract	Conductive rubber nanocomposites were prepared by dispersing conductive nanotubes (CNT) in thermoreversibly cross-linked ethylene propylene rubbers grafted with furan groups (EPM-g-furan) rubbers. Their features were studied with a strong focus on conductive and mechanical properties relevant for strain-sensor applications. The Diels-Alder chemistry used for thermoreversible cross-linking allows for the preparation of fully recyclable, homogeneous, and conductive nanocomposites. CNT modified with compatible furan groups provided nanocomposites with a relatively large tensile strength and small elongation at break. High and low sensitivity deformation experiments of nanocomposites with 5 wt % CNT (at the percolation threshold) displayed an initially linear sensitivity to deformation. Notably, only fresh samples displayed a linear response of their electrical resistivity to deformations as the resistance variation collapsed already after one cycle of elongation. Notwithstanding this mediocre performance as a strain sensor, the advantages of using thermoreversible chemistry in a conductive rubber nanocomposite were highlighted by demonstrating crack-healing by welding due to the joule effect on the surface and the bulk of the material. This will open up new technological opportunities for the design of novel strain-sensors based on recyclable rubbers.
e-ISSN	20794991
DOI	10.3390/nano8020058
Journal	Nanomaterials
Issue Number	2
Volume Number	8
Language	English
Publisher	MDPI AG
Publisher Date	2018-01-01
Publisher Place	Switzerland
Access Restriction	Open
Subject Keyword	Chemistry Crack-healing Strain Sensor Rubber Nanocomposite Thermoreversible Cross-linking Joule Effect
Content Type	Text
Resource Type	Article

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