NDLI: A Polysulfide-Infiltrated Carbon Cloth Cathode for High-Performance Flexible Lithium

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A Polysulfide-Infiltrated Carbon Cloth Cathode for High-Performance Flexible Lithium–Sulfur Batteries

Content Provider	Directory of Open Access Journals (DOAJ)
Author	Ji-Yoon Song Hyeon-Haeng Lee Won Gi Hong Yun Suk Huh Yun Sung Lee Hae Jin Kim Young-Si Jun
Abstract	For practical application of lithium–sulfur batteries (LSBs), it is crucial to develop sulfur cathodes with high areal capacity and cycle stability in a simple and inexpensive manner. In this study, a carbon cloth infiltrated with a sulfur-containing electrolyte solution (CC-S) was utilized as an additive-free, flexible, high-sulfur-loading cathode. A freestanding carbon cloth performed double duty as a current collector and a sulfur-supporting/trapping material. The active material in the form of Li2S6 dissolved in a 1 M LiTFSI-DOL/DME solution was simply infiltrated into the carbon cloth (CC) during cell fabrication, and its optimal loading amount was found to be in a range between 2 and 10 mg/cm2 via electrochemical characterization. It was found that the interwoven carbon microfibers retained structural integrity against volume expansion/contraction and that the embedded uniform micropores enabled a high loading and an efficient trapping of sulfur species during cycling. The LSB coin cell employing the CC-S electrode with an areal sulfur loading of 6 mg/cm2 exhibited a high areal capacity of 4.3 and 3.2 mAh/cm2 at C/10 for 145 cycles and C/3 for 200 cycles, respectively, with minor capacity loss (<0.03%/cycle). More importantly, such high performance could also be realized in flexible pouch cells with dimensions of 2 cm × 6 cm before and after 300 bending cycles. Simple and inexpensive preparation of sulfur cathodes using CC-S electrodes, therefore, has great potential for the manufacture of high-performance flexible LSBs.
e-ISSN	20794991
DOI	10.3390/nano8020090
Journal	Nanomaterials
Issue Number	2
Volume Number	8
Language	English
Publisher	MDPI AG
Publisher Date	2018-01-01
Publisher Place	Switzerland
Access Restriction	Open
Subject Keyword	Chemistry Lithium–sulfur Batteries Flexible Batteries Carbon Cloth Microporous Carbon Catholytes
Content Type	Text
Resource Type	Article

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