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| Content Provider | World Health Organization (WHO)-Global Index Medicus |
|---|---|
| Author | Bulychev, V. P. Schepkin, D. N. Bulanin, Capital Ka Cyrillic Ð Herrebout, W. |
| Description | Author Affiliation: Bulanin CK ( Department of Physics, St.- Petersburg State University, Peterhof, St. Petersburg 198504, Russia. Electronic address: kbulanin@mail.ru.) |
| Abstract | Infrared spectra are reported of ozone and HCl dissolved in liquid argon (86-134 K) at concentrations varying from 5×10(-5) to 9×10(-6) M for HCl, and from 1×10(-3) to 5×10(-5) M for ozone. At low concentrations of O3 and of HCl, no spectral features due to O3-HCl complex were found. At higher concentrations (1×10(-3) of ozone vs 5×10(-5)-9×10(-6) of HCl), a new band near 2840 cm(-1) due to the HCl···O3 complex was observed. FWHM of νHCl of the complex is 8 cm(-1). From the temperature dependence of the absorption band intensity, the enthalpy of the complex formation was estimated, ΔH°=4.7±0.4 kJ mole(-1). The optimized geometry of the cis-HCl···O3 complex and a value of 6.3 kJ mole(-1) for its binding energy were determined by ab initio calculations. |
| ISSN | 13861425 |
| Volume Number | 117 |
| e-ISSN | 18733557 |
| Journal | Spectrochimica Acta Part A: Molecular and Biomolecular Spectroscopy |
| Language | English |
| Publisher | Elsevier |
| Publisher Date | 2014-01-03 |
| Publisher Place | Great Britain (UK) |
| Access Restriction | One Nation One Subscription (ONOS) |
| Subject Keyword | Argon Chemistry Hydrochloric Acid Ozone Computer Simulation Solvents Spectrophotometry, Infrared Thermodynamics Journal Article Research Support, Non-u.s. Gov't Discipline Spectroscopy |
| Content Type | Text |
| Resource Type | Article |
| Subject | Spectroscopy Atomic and Molecular Physics, and Optics Analytical Chemistry Instrumentation |
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