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| Content Provider | World Health Organization (WHO)-Global Index Medicus |
|---|---|
| Author | Holldack, Karsten Tregenna-piggott, Philip Weihe, Høgni Bendix, Jesper Waldmann, Oliver Dreiser, Jan Schau-magnussen, Magnus Schnegg, Alexander Pedersen, Kasper S. Nehrkorn, Joscha Mutka, Hannu |
| Description | Author Affiliation: Dreiser J ( Physikalisches Institut, Universität Freiburg, 79104 Freiburg, Germany. jan.dreiser@psi.ch) |
| Abstract | We have investigated the novel single-molecule magnet $(NEt_{4})[Mn_{2}(5-Brsalen)_{2}(MeOH)_{2}Cr(CN)_{6}]$ (1; 5-Brsalen=N,N′-ethylenebis(5-bromosalicylidene)iminato anion) using spectroscopic as well as magnetization and susceptibility measurements. Frequency-domain Fourier-transform terahertz electron paramagnetic resonance (FDFT THz-EPR) based on the generation of THz radiation from a synchrotron in combination with inelastic neutron scattering (INS) allows for the discrimination between intermultiplet and intramultiplet transitions. Together with ac/dc magnetic susceptibility measurements the obtained set of data provides a complete characterization of the lowest energetic magnetic excitations. We find that the new compound 1 exhibits much weaker intermolecular interactions than found in the closely related compound: $K[Mn_{2}(5-Brsalen)_{2}(H_{2}O)_{2}Cr(CN)_{6}]$ (2). Furthermore, two phonon lines in the vicinity of the magnetic excitations are detected. |
| ISSN | 09476539 |
| e-ISSN | 15213765 |
| Journal | Chemistry - A European Journal |
| Issue Number | 27 |
| Volume Number | 17 |
| Language | English |
| Publisher | Wiley-VCH;ChemPubSoc Europe |
| Publisher Date | 2011-06-27 |
| Publisher Place | Germany |
| Access Restriction | Open |
| Subject Keyword | Chemistry |
| Content Type | Text |
| Resource Type | Article |
| Subject | Organic Chemistry Catalysis |
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