NDLI: Rational design of anode materials based on GroupâIVA elements (Si, Ge, and Sn) for lithium-ion batteries.

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Rational design of anode materials based on GroupâIVA elements (Si, Ge, and Sn) for lithium-ion batteries.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Wu, Xing-Long Guo, Yu-Guo Wan, Li-Jun
Description	Author Affiliation: Wu XL ( CAS Key Laboratory of Molecular Nanostructure and Nanotechnology, Institute of Chemistry, Chinese Academy of Sciences (CAS), Beijing, 100190, PR China.)
Abstract	Lithium-ion batteries (LIBs) represent the state-of-the-art technology in rechargeable energy-storage devices and they currently occupy the prime position in the marketplace for powering an increasingly diverse range of applications. However, the fast development of these applications has led to increasing demands being placed on advanced LIBs in terms of higher energy/power densities and longer life cycles. For LIBs to meet these requirements, researchers have focused on active electrode materials, owing to their crucial roles in the electrochemical performance of batteries. For anode materials, compounds based on GroupâIVA (Si, Ge, and Sn) elements represent one of the directions in the development of high-capacity anodes. Although these compounds have many significant advantages when used as anode materials for LIBs, there are still some critical problems to be solved before they can meet the high requirements for practical applications. In this Focus Review, we summarize a series of rational designs for GroupâIVA-based anode materials, in terms of their chemical compositions and structures, that could address these problems, that is, huge volume variations during cycling, unstable surfaces/interfaces, and invalidation of transport pathways for electrons upon cycling. These designs should at least include one of the following structural benefits: 1)âContain a sufficient number of voids to accommodate the volume variations during cycling; 2)âadopt a 'plum-pudding'-like structure to limit the volume variations during cycling; 3)âfacilitate an efficient and permanent transport pathway for electrons and lithium ions; or 4)âshow stable surfaces/interfaces to stabilize the inâsitu formed SEI layers.
File Format	HTM / HTML
ISSN	18614728
Issue Number	9
Journal	Chemistry - An Asian Journal
Volume Number	8
e-ISSN	1861471X
Language	English
Publisher	Wiley-VCH
Publisher Date	2013-09-01
Publisher Place	Germany
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Discipline Chemistry
Content Type	Text
Resource Type	Article
Subject	Organic Chemistry Biochemistry

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Rational design of anode materials based on Groupâ IVA elements (Si, Ge, and Sn) for lithium-ion batteries.

Rational design of anode materials based on GroupâIVA elements (Si, Ge, and Sn) for lithium-ion batteries.