NDLI: Influence of intermolecular forces at critical-point wedge filling.

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Influence of intermolecular forces at critical-point wedge filling.

Content Provider	World Health Organization (WHO)-Global Index Medicus
Author	Malijevský, Alexandr Parry, Andrew O.
Description	Country affiliation: Czech Republic Author Affiliation: Malijevský A ( Department of Physical Chemistry, Institute of Chemical Technology, Prague, 166 28 Praha 6, Czech Republic and Institute of Chemical Process Fundamentals, Academy of Sciences, 16502 Prague 6, Czech Republic.); Parry AO ( Department of Mathematics, Imperial College London, London SW7 2B7, United Kingdom.)
Abstract	We use microscopic density functional theory to study filling transitions in systems with long-ranged wall-fluid and short-ranged fluid-fluid forces occurring in a right-angle wedge. By changing the strength of the wall-fluid interaction we can induce both wetting and filling transitions over a wide range of temperatures and study the order of these transitions. At low temperatures we find that both wetting and filling transitions are first order in keeping with predictions of simple local effective Hamiltonian models. However close to the bulk critical point the filling transition is observed to be continuous even though the wetting transition remains first order and the wetting binding potential still exhibits a small activation barrier. The critical singularities for adsorption for the continuous filling transitions depend on whether retarded or nonretarded wall-fluid forces are present and are in excellent agreement with predictions of effective Hamiltonian theory even though the change in the order of the transition was not anticipated.
File Format	HTM / HTML
ISSN	24700045
e-ISSN	24700053
Journal	Physical Review E
Volume Number	93
Language	English
Publisher	American Physical Society
Publisher Date	2016-04-01
Publisher Place	United States
Access Restriction	Open
Subject Keyword	Statistical and Nonlinear Physics many-body systems Condensed Matter Physics
Content Type	Text
Resource Type	Article
Subject	Statistics and Probability Statistical and Nonlinear Physics Condensed Matter Physics

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