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The effect of synthesis method and post-synthesis treatment on the formation of neutral Mn(II) complex into anionic zeolite structure and investigation of its catalytic activity in the epoxidation of alkenes

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The effect of synthesis method and post-synthesis treatment on the formation of neutral Mn(II) complex into anionic zeolite structure and investigation of its catalytic activity in the epoxidation of alkenes

Content Provider	Springer Nature Link
Author	Alemi, Abdolali Marefat, Mohammad Reza Moosavifar, Maryam Mahmoodi, Hossein Nouruzi, Nasrin
Copyright Year	2014
Abstract	In this study, we improved the catalytic performance of manganese porphyrin encapsulated HY zeolite for alkene epoxidation reaction. For this purpose, Manganese tetra pyridyl porphyrin encapsulated into modified dealuminated Y zeolite (MnTPP-MDAZY) was synthesized using zeolite template synthesis method. This heterogenized catalyst was characterized by FT-IR, UV–Vis, XRD and atomic absorption spectra (AAS) technique. Catalyst loading was 0.263 mmol/g support. In this way, high catalyst loading is probably related to the decrease of the size of metalloporphyrin and the post-synthesis treatment. The latter one causes the increase of the diameter of the mesoporous structure as a result of the dealumination of zeolite with EDTA treatment. High catalyst loading efficiently enhances the epoxidation of alkenes.
Starting Page	1561
Ending Page	1567
Page Count	7
File Format	PDF
ISSN	1735207X
Journal	Journal of the Iranian Chemical Society
Volume Number	11
Issue Number	6
e-ISSN	17352428
Language	English
Publisher	Springer Berlin Heidelberg
Publisher Date	2014-04-03
Publisher Place	Berlin, Heidelberg
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Analytical Chemistry Manganese porphyrin Catalyst loading Zeolite template synthesis Physical Chemistry Dealuminated zeolite Y Alkene epoxidation Biochemistry Inorganic Chemistry Organic Chemistry
Content Type	Text
Resource Type	Article
Subject	Chemistry

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The effect of synthesis method and post-synthesis treatment on the formation of neutral Mn(II) complex into anionic zeolite structure and investigation of its catalytic activity in the epoxidation of alkenes

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The effect of synthesis method and post-synthesis treatment on the formation of neutral Mn(II) complex into anionic zeolite structure and investigation of its catalytic activity in the epoxidation of alkenes

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