NDLI: Optical characterization of CDOM in a marsh-influenced environment in the Changjiang (Yangtze River) Estuary

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Optical characterization of CDOM in a marsh-influenced environment in the Changjiang (Yangtze River) Estuary

Content Provider	Springer Nature Link
Author	Gao, Lei Fan, Daidu Sun, Chengxing Li, Daoji Cai, Jingong
Copyright Year	2010
Abstract	To elucidate the influence of tidal marshes on the amount and chemical structure of chromophoric dissolved organic matter (CDOM) in adjacent coastal waters, surface water samples were collected along three cross-marsh transects in tidal marshes within the Changjiang Estuary. In addition, three sediment cores were collected from the marshes and incubated for 10 h in the laboratory after adding overlying tidal waters. Nutrients, DOC, absorption, fluorescence excitation–emission matrix (EEM) spectroscopy, and other parameters were measured in these samples, which clearly illustrated releases by the tidal marshes of DOC, and CDOM absorbent and fluorescent molecules. To characterize the chemical nature of the marsh-derived CDOM, variations in a suite of optical indices (including molar absorptivity, absorption spectral slope, fluorescence quantum yield, and fluorescence ratios between certain excitation/emission locations) in these samples were plotted against the offshore distance of the stations as well as the incubation time. From the literature, it has been suggested that these variations are closely associated with molecular weight, aromaticity, and humic/fulvic or allochthonous/autochthonous ratios in the CDOM mixtures. This study showed that the CDOM fluorophores changed to more humic-like and were less protein-like from sea to land across the marsh gradients. Furthermore, subtractions between EEM spectra before and after laboratory incubations were applied to illustrate in greater detail the properties of the pure fluorescent compounds exchanged at the sediment–overlying water interface.
Starting Page	643
Ending Page	658
Page Count	16
File Format	PDF
ISSN	18666280
Journal	Environmental Earth Sciences
Volume Number	64
Issue Number	3
e-ISSN	18666299
Language	English
Publisher	Springer-Verlag
Publisher Date	2010-12-12
Publisher Place	Berlin, Heidelberg
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Chromophoric dissolved organic matter Light absorption Fluorescence spectroscopy Sediment–water exchanges Salt marshes Changjiang (Yangtze River) Estuary Geology
Content Type	Text
Resource Type	Article
Subject	Global and Planetary Change Earth-Surface Processes Soil Science Environmental Chemistry Pollution Geology Water Science and Technology

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