NDLI: 3-Aminopropyltriethoxysilane-Assisted Si@SiO$_{2}$/CNTs Hybrid Microspheres as Superior Anode Materials for Li-ion Batteries

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3-Aminopropyltriethoxysilane-Assisted Si@SiO$_{2}$/CNTs Hybrid Microspheres as Superior Anode Materials for Li-ion Batteries

Content Provider	Springer Nature Link
Author	Wang, Jiyun Hou, Xianhua Zhang, Miao Li, Yana Wu, Yuping Liu, Xiang Hu, Shejun
Copyright Year	2016
Abstract	A silicon based composite (Si@SiO$_{2}$/CNTs) with outstanding electrochemistry performance has been easily synthesized using a spray drying method; The composite microsphere is mainly made up of carbon nanotubes and the prepared nano silicon particles. With the help of a silane coupling agent, carbon nanotubes tightly intertwined with nano silicon particles and formed microspheres together. On the surface of the prepared nano silicon particles, a layer of oxide film plays a role as a barrier to reduce the rupture of the particles during the lithium intercalation/extraction process. In addition, the added twisted carbon nanotubes can help to maintain the conductive network, thus stabilizing the electrode working environment during the lithium intercalation/extraction process. As a superior anode material, an initial specific discharge capacity of approximately 2846.9 mAh g$^{−1}$ with a coulombic efficiency of 86 % and a reversible specific capacity of 2035.9 mAh g$^{−1}$ after 100 cycles at a constant density of 500 mA g$^{−1}$ are obtained.
Starting Page	97
Ending Page	104
Page Count	8
File Format	PDF
ISSN	1876990X
Journal	Silicon
Volume Number	9
Issue Number	1
e-ISSN	18769918
Language	English
Publisher	Springer Netherlands
Publisher Date	2016-04-12
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Silicon Composites Electronic materials Li-ion batteries Inorganic Chemistry Materials Science Optics, Lasers, Photonics, Optical Devices Environmental Chemistry
Content Type	Text
Resource Type	Article
Subject	Electronic, Optical and Magnetic Materials

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