NDLI: Investigation of the deterioration of passive films in H$

Content Provider	Springer Nature Link
Author	Wang, Zhu Zhang, Lei Tang, Xian Cui, Zhao yang Xue, Jun peng Lu, Min xu
Copyright Year	2016
Abstract	The effect of H$_{2}$S on the corrosion behavior of 316L stainless steel was investigated using electrochemical methods by changing the gas condition from CO$_{2}$ to H$_{2}$S and then back to CO$_{2}$. The presence of H$_{2}$S showed an acceleration effect on the corrosion of 316L stainless steel in comparison with CO$_{2}$. The acceleration effect remained even after the complete removal of H$_{2}$S by CO$_{2}$, indicating that the passive film was irreversibly damaged. X-ray photoelectron spectroscopy (XPS) analysis indicated that the passive film was composed of Cr$_{2}$O$_{3}$, Fe$_{2}$O$_{3}$, and FeS$_{2}$ after being immersed in H$_{2}$S-containing solutions. The semiconducting property of the passive film was then investigated by using the Mott–Schottky approach. The presence of sulfides resulted in higher acceptor and donor densities and thus was responsible for the deterioration of passive films.
Starting Page	943
Ending Page	953
Page Count	11
File Format	PDF
ISSN	16744799
Journal	International Journal of Minerals, Metallurgy, and Materials
Volume Number	24
Issue Number	8
e-ISSN	1869103X
Language	English
Publisher	University of Science and Technology Beijing
Publisher Date	2017-07-29
Publisher Place	Beijing
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	stainless steel passive films hydrogen sulfide corrosion Materials Science Metallic Materials Characterization and Evaluation of Materials Ceramics, Glass, Composites, Natural Materials Surfaces and Interfaces, Thin Films Tribology, Corrosion and Coatings
Content Type	Text
Resource Type	Article
Subject	Materials Chemistry Mechanics of Materials Metals and Alloys Geochemistry and Petrology Mechanical Engineering

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