NDLI: Basic principles of ultrafast Raman loss spectroscopy$^{#}$

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Basic principles of ultrafast Raman loss spectroscopy$^{#}$

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Basic principles of ultrafast Raman loss spectroscopy$^{#}$

Content Provider	Springer Nature Link
Author	RAI, N K LAKSHMANNA, A Y NAMBOODIRI, V V
Copyright Year	2012
Abstract	When a light beam passes through any medium, the effects of interaction of light with the material depend on the field intensity. At low light intensities the response of materials remain linear to the amplitude of the applied electromagnetic field. But for sufficiently high intensities, the optical properties of materials are no longer linear to the amplitude of applied electromagnetic field. In such cases, the interaction of light waves with matter can result in the generation of new frequencies due to nonlinear processes such as higher harmonic generation and mixing of incident fields. One such nonlinear process, namely, the third order nonlinear spectroscopy has become a popular tool to study molecular structure. Thus, the spectroscopy based on the third order optical nonlinearity called stimulated Raman spectroscopy (SRS) is a tool to extract the structural and dynamical information about a molecular system. Ultrafast Raman loss spectroscopy (URLS) is analogous to SRS but is more sensitive than SRS. In this paper, we present the theoretical basis of SRS (URLS) techniques which have been developed in our laboratory. Graphical Abstract The fundamentals of non-linear optical spectroscopy are presented. The theory is extended to understand the third order non-linear Raman spectroscopic techniques named as stimulated Raman spectroscopies. A systematic method to describe the Ultrafast Raman loss spectroscopy (URLS), a third ordered nonlinear Raman process, is also presented.
Starting Page	177
Ending Page	186
Page Count	10
File Format	PDF
ISSN	09743626
Journal	Journal of Chemical Sciences
Volume Number	124
Issue Number	1
e-ISSN	09737103
Language	English
Publisher	Springer-Verlag
Publisher Date	2012-03-21
Publisher Institution	Indian Academy of Sciences
Publisher Place	India
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Nonlinear spectroscopy phase matching condition third order nonlinear process SRS URLS Chemistry/Food Science
Content Type	Text
Resource Type	Article
Subject	Chemistry

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