NDLI: The capture of carbon dioxide by transition metal aluminates, calcium aluminate, calcium zirconate, calcium silicate and lithium zirconate

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Frontiers of Chemical Engineering in China : Volume 5, Issue 3, September 2011

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The capture of carbon dioxide by transition metal aluminates, calcium aluminate, calcium zirconate, calcium silicate and lithium zirconate

Content Provider	Springer Nature Link
Author	Tilekar, Ganesh Shinde, Kiran Kale, Kishor Raskar, Reshma Gaikwad, Abaji
Copyright Year	2011
Abstract	The capture of CO$_{2}$ by transition metal (Mn, Ni, Co and Zn) aluminates, calcium aluminate, calcium zirconate, calcium silicate and lithium zirconate was carried out at pre- and post-combustion temperatures. The prepared metal adsorbents were characterized by Xray diffraction (XRD), scanning electron microscope (SEM), surface area analysis and acidity/alkalinity measurements. The different experimental variables affecting the adsorbents ability to capture CO$_{2}$, such as the mol ratio of metal ions, the pressure of CO$_{2}$, the exposure time and the temperature of the adsorbent were also investigated. Calcium zirconate captured 13.85 wt-% CO$_{2}$ at 650°C and 2.5 atm and calcium silicate captured 14.31 wt-%at 650°C. Molecular sieves (13X) and carbon can only capture a negligible amount of CO$_{2}$ at high temperatures (300°C–650°C). However, the mixed metal oxides captured reasonable amount of CO$_{2}$ at these higher temperatures. In addition, calcium aluminate, calcium zirconate, calcium silicate and lithium zirconate adsorbents captured CO$_{2}$ at both pre and post-combustion temperatures. The trend for the amount of captured carbon dioxide over the adsorbents was calcium aluminate < lithium zirconate < calcium zirconate < calcium silicate.
Starting Page	477
Ending Page	491
Page Count	15
File Format	PDF
ISSN	20950179
Journal	Frontiers of Chemical Engineering in China
Volume Number	5
Issue Number	4
e-ISSN	16737474
Language	English
Publisher	SP Higher Education Press
Publisher Date	2011-11-04
Publisher Institution	Chinese Universities
Publisher Place	Heidelberg
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	captured CO$_{2}$ pre-combustion temperature characterization calcium silicate calcium zirconate Industrial Chemistry/Chemical Engineering Nanotechnology
Content Type	Text
Resource Type	Article
Subject	Chemical Engineering

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