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The heats of exchange of transition metal ions on the Na form of clinoptilolite

Content Provider	Springer Nature Link
Author	Tarasevich, Yu. I. Krysenko, D. A. Polyakov, V. E. Aksenenko, E. V.
Copyright Year	2008
Abstract	Direct calorimetric measurements were used to determine the heats of exchange of the Mn$^{2+}$, Co$^{2+}$, Cu$^{2+}$, and Ni$^{2+}$ cations on the Na form of clinoptilolite over the entire range of solid phase fillings with sorbed cations. In parallel, ion exchange isotherms for the systems were measured by the sorption-analytic method. The integral free energies and entropies of ion exchange were calculated. It was shown that the solution phase of the clinoptilolite-electrolyte solution two-phase system contributed significantly to the total thermodynamic characteristics of ion exchange. The differentiation of the dependence of the integral enthalpy on the degree of filling was performed to show that the clinoptilolite structure contained at least two types of exchange sites having different interaction energies with transition metal ions.
Starting Page	1506
Ending Page	1511
Page Count	6
File Format	PDF
ISSN	00360244
Journal	Russian Journal of Physical Chemistry
Volume Number	82
Issue Number	9
e-ISSN	1531863X
Language	English
Publisher	SP MAIK Nauka/Interperiodica
Publisher Date	2008-08-22
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Physical Chemistry
Content Type	Text
Resource Type	Article
Subject	Physical and Theoretical Chemistry

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