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Effect the conditions of the acid–thermal modification of clinoptilolite have on the catalytic properties of palladium–copper complexes anchored on it in the reaction of carbon monoxide oxidation

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Effect the conditions of the acid–thermal modification of clinoptilolite have on the catalytic properties of palladium–copper complexes anchored on it in the reaction of carbon monoxide oxidation

Content Provider	Springer Nature Link
Author	Rakitskaya, T. L. Kiose, T. A. Ennan, A. A. Golubchik, K. O. Oleksenko, L. P. Gerasiova, V. G.
Copyright Year	2016
Abstract	The dependence of the physicochemical and structural–adsorption properties of natural and acid–thermal modified clinoptilolite, and of Pd(II)–Cu(II) catalysts based on them, on the duration of acid–thermal modification is investigated. The samples under study are described via XRD and thermal gravimetric (DTG and DTA) analysis, IR, DR UV–Vis, EPR spectroscopy, and water vapor adsorption. Values of both the specific surface area (S $_{sp}$) and pH of aqueous suspensions are determined. The resulting catalysts are tested in the reaction of low-temperature carbon monoxide oxidation with air oxygen. A conclusion is drawn about the nature of surface bimetallic Pd(II)–Cu(II) complexes. The greatest catalytic activity is shown by complexes based on clinoptilolite and modified with 3 M HNO$_{3}$ for 0.5 and 1 h.
Starting Page	1120
Ending Page	1127
Page Count	8
File Format	PDF
ISSN	00360244
Journal	Russian Journal of Physical Chemistry
Volume Number	90
Issue Number	6
e-ISSN	1531863X
Language	English
Publisher	Pleiades Publishing
Publisher Date	2016-05-21
Publisher Place	Moscow
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	clinoptilolite carbon monoxide oxidation catalyst palladium(II) copper(II) XRD thermogravimetric analysis IR DR UV–Vis EPR spectroscopy Physical Chemistry
Content Type	Text
Resource Type	Article
Subject	Physical and Theoretical Chemistry

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