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SHG from centrosymmetric supermolecular crystal

Content Provider	Springer Nature Link
Author	Wensheng, Guo Guo, Fang Wei, Chunsheng Liu, Qitao Zhou, Guangyong Wang, Dong Shao, Zhongshu
Copyright Year	2002
Abstract	Supermolecular crystal composed of p-nitrophenol, hexamethylenetetramine, phosphoric acid and water was obtained by supermolecular assembly. The crystal has a centrosymmetric structure with space group P2$_{1}$/c. The relative intensity and integral value of green frequency doubling of light from the crystal powder compared with that from KDP powder measured by pico-second Nd:YAG laser are 757.3 (KDP: 183.4) and 1771.7 (KDP: 423.98), respectively. In supermolecular crystal, due to the arrangement of centrosymmetric p-nitrophenol molecules in the inorganic-organic host framework formed by hexamethylenetetramine, phosphoric acid and water, the distances between the p-nitrophenol molecules with centrosymmetry are changed (N1A-O1A: 0.8158 nm, N1B’-O1B: 1.4450 nm, N1A-N1A’: 0.5837 nm, N1B’-N1B: 0.6898 nm), and the interaction between the dipoles becomes weak, which is easy for the ground state to turn into the excited state charge separated form, and generate the stable asymmetrical distribution of π-electron cloud density of quinonal structure, thus exhibiting SHG effect.
Starting Page	267
Ending Page	274
Page Count	8
File Format	PDF
ISSN	10069291
Journal	Science in China Series B: Chemistry
Volume Number	45
Issue Number	3
e-ISSN	18622771
Language	English
Publisher	Science in China Press
Publisher Date	2002-01-01
Publisher Place	Beijing
Access Restriction	Subscribed
Subject Keyword	supermolecular crystal SHG effect centrosymmetry p-nitrophenol Chemistry/Food Science
Content Type	Text
Resource Type	Article
Subject	Chemistry

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