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| Content Provider | Springer Nature Link |
|---|---|
| Author | Appleby, P. G. |
| Copyright Year | 1997 |
| Abstract | The fallout radionuclides$^{210}$Pb and$^{137}$Cs are widely used to date environmental records contained in lake sediments. Since the radionuclide records are themselves the outcome of the transformation of atmospheric fallout by mediating transport processes from the catchment, through the water column and post-depositional migration via pore waters, reliable models of these processes are crucial to accurate dating. The large quantities of data on$^{210}$Pb and$^{137}$Cs in lake sediments accumulated through their widespread dating applications may be used to study transport models. Their advantages as tracers of transport processes include widespread dispersal through the environment, relatively simple and well known input functions, and ease of measurement.One of the principle factors controlling the transport of any species through the water column is its distribution between aqueous and particulate phases. The relatively solubility of$^{137}$Cs in the water column is demonstrated by the reduced$^{137}$Cs,$^{210}$Pb inventory ratios in sediments compared to values expected from direct fallout. Using sediment records from a wide range of Cumbrian lakes, calculations based on simple models indicate that the particulate fraction of weapons fallout$^{137}$Cs in the water column ranged from 5–22%, and was proportional to the square root of the sedimentation rate (determined by$^{210}$Pb). TheK $_{D}$ value for weapons$^{137}$Cs in the water column is estimated to be in the range 1–2×10$^{5}$ L kg$^{−1}$. This is comparable withK $_{D}$ values for Chernobyl$^{137}$Cs in these lakes (Smithet al. in press) obtained from direct measurements in the cater column. |
| Starting Page | 573 |
| Ending Page | 585 |
| Page Count | 13 |
| File Format | |
| ISSN | 00496979 |
| Journal | Water, Air, and Soil Pollution |
| Volume Number | 99 |
| Issue Number | 1-4 |
| e-ISSN | 15732932 |
| Language | English |
| Publisher | Kluwer Academic Publishers |
| Publisher Date | 1997-01-01 |
| Publisher Place | Dordrecht |
| Access Restriction | One Nation One Subscription (ONOS) |
| Subject Keyword | sedimentation rates lead-210 cesium-137 particulate phase Hydrogeology Environment Atmospheric Protection/Air Quality Control/Air Pollution Terrestrial Pollution Waste Water Technology Water Pollution Control Water Management Aquatic Pollution |
| Content Type | Text |
| Resource Type | Article |
| Subject | Ecological Modeling Environmental Chemistry Pollution Environmental Engineering Water Science and Technology |
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