NDLI: Atmospheric Concentration of Ammonia, Nitrogen Dioxide, Nitric Acid, and Sulfur Dioxide by Passive Method within Osaka Prefecture and Their Emission Inventory

Content Provider	Springer Nature Link
Author	Nishikawa, Yoshiri Kannari, Akiyoshi
Copyright Year	2010
Abstract	Annual emission map for NH$_{3}$, NO$_{X}$, and SO$_{2}$ within Osaka prefecture was shown according to the EAGrid2000-Japan emission database. The median emission of NH$_{3}$, NO$_{X}$, and SO$_{2}$ was 1.94, 24.8, 1.32 ton/km$^{2}$/year, respectively, while that at 11 passive sampling sites was 1.61, 17.3, 0.74 ton/km$^{2}$/year, respectively. Monthly emission for NH$_{3}$ showed apparent seasonal trends, being high in summer and low in winter. That for NO$_{X}$ and SO$_{2}$ was slightly high in winter and low in summer and constant through the year, respectively. Atmospheric concentration of NH$_{3}$, NO$_{2}$, HNO$_{3}$, and SO$_{2}$ by the passive method was compared with corresponding emission inventory. Average concentrations of HNO$_{3}$, SO$_{2}$, NH$_{3}$, and NO$_{2}$ in June were 16–67, 23–135, 21–173, and 149–873 nmol/m$^{3}$, respectively, while those in October were 5–21, 16–72, 14–196, and 169–1,167 nmol/m$^{3}$, respectively. The emission inventory flux of SO$_{2}$, NO$_{X}$, and NH$_{3}$ was calculated both within 1 × 1- and 3 × 3-km mesh. It was a small difference between June and October for SO$_{2}$ and NO$_{X}$ in the both meshes. For NH$_{3}$, emission flux in June was around twofold of that in October. The NH$_{3}$ correlation between concentration and emission flux was excellent in the 1 × 1 km mesh, although somewhat decreased in the 3 × 3 km mesh. In the case of NO$_{2}$, the correlation for the 3 × 3 km mesh, however, was more increased than the 1 × 1 km mesh. The correlation for HNO$_{3}$ and SO$_{2}$ was a small difference with the both meshes. Monthly concentrations of NH$_{3}$, NO$_{2}$, HNO$_{3}$, and SO$_{2}$ were compared with their corresponding gases emission at whole-year survey sites. Concentration of NH$_{3}$ was high from July to November, while emission of NH$_{3}$ was high from June to September (summer) and low from December to March (winter). Trend of NO$_{2}$ concentration was high in winter and low in summer, a similar tendency to that of NO$_{X}$ emission. On the other hand, the trend of HNO$_{3}$ concentration was high in summer and low in winter. There was no particular seasonal trend of SO$_{2}$ concentration and SO$_{2}$ emission had also no seasonal variation but was constant.
Starting Page	229
Ending Page	237
Page Count	9
File Format	PDF
ISSN	00496979
Journal	Water, Air, and Soil Pollution
Volume Number	215
Issue Number	1-4
e-ISSN	15732932
Language	English
Publisher	Springer Netherlands
Publisher Date	2010-05-19
Publisher Place	Dordrecht
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Emission inventory Third-order mesh code Passive method NH$_{3}$ NO$_{2}$ NO$_{X}$ HNO$_{3}$ SO$_{2}$ Climate Change Hydrogeology Soil Science & Conservation Waste Water Technology Water Pollution Control Water Management Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution Environment
Content Type	Text
Resource Type	Article
Subject	Ecological Modeling Environmental Chemistry Pollution Environmental Engineering Water Science and Technology

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