NDLI: The Synthesis and Photocatalytic Properties of Nitrogen Doped TiO$_{2}$ Films Prepared Using the AC-PLD Method

Content Provider	Springer Nature Link
Author	Sato, buaki Matsuda, Miru Yoshinaga, Masaki Nakamura, Takahiro Sato, Shunichi Muramatsu, Atsushi
Copyright Year	2009
Abstract	Synthesis of N doped TiO$_{2}$ films were conducted by the atmospheric controlled pulsed laser deposition (AC-PLD) method to generate visible light active photocatalytic films. In this method, the anion doped TiO$_{2}$ films were synthesized on a quartz substrate by the irradiation of a pulsed Nd:YAG laser on a TiO$_{2}$ target in the presence of gaseous nitrogen containing reagents at reduced pressure. For nitrogen doping, the use of CH$_{3}$CN was found to be more effective than the use of NH$_{3}$. The visible light absorption properties of the films were very sensitive to the CH$_{3}$CN partial pressure during ablation. When using CH$_{3}$CN, nitrogen and an equal quantity of carbon was uniformly doped into the TiO$_{2}$ films. The resultant films showed better catalytic performance than those which were either un-doped or doped using NH$_{3}$. The formation of nitrogen doped TiO$_{2}$ is discussed by relating experimental results to thermodynamic considerations. It is also suggested that stronger reducing agents such as carbon are required for doping nitrogen into TiO$_{2}$ films.
Starting Page	1592
Ending Page	1597
Page Count	6
File Format	PDF
ISSN	10225528
Journal	Topics in Catalysis
Volume Number	52
Issue Number	11
e-ISSN	15729028
Language	English
Publisher	Springer US
Publisher Date	2009-04-28
Publisher Place	Boston
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	Titanium dioxide Nitrogen doping AC-PLD Photocatalyst Characterization and Evaluation of Materials Industrial Chemistry/Chemical Engineering Pharmacy Physical Chemistry Catalysis
Content Type	Text
Resource Type	Article
Subject	Chemistry Catalysis

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