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Silicon carbide nanotubes and nanotubular fibers: Synthesis, stability, structure, and classification

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Silicon carbide nanotubes and nanotubular fibers: Synthesis, stability, structure, and classification

Content Provider	Springer Nature Link
Author	Pokropivnyi, V. V. Silenko, P. M.
Copyright Year	2006
Abstract	Published data on silicon carbide nanotubes (SiC-NT) are analyzed. According to theoretical calculations, single-layer SiC-NTs do not dissociate, but they have not yet been detected experimentally. According to the experimental data, metastable SiC-NTs with walls consisting of several layers and nanotube fibers were produced. The optimized structure of single-layer SiC-NTs was calculated by the RHF/6-31G quantum-chemical method. The possibility of obtaining SiC-NTs by gas-phase chemical deposition from methyltrichlorosilane in the temperature range of 800–1000 °C was investigated. Nanofibers and polygrained SiC nanotubes were obtained, but ordinary layer SiC nanotubes were not detected. To remove the inconsistencies it was first proposed to classify the nanotubes according to the structure of their walls, separating all the SiC-NTs into three types: 1) ordinary layer nanotubes with rolled layers, similar to carbon nanotubes; 2) polynanocrystalline nanotubular fibers or nanotubes with walls consisting of linked differently oriented nanograins; 3) monocrystalline synthetic nanotubes with ideal crystalline walls. It was concluded that the ordinary SiC-NTs of the first type are unstable with the exception of one-or two-layer nanotubes; stable SiC-NTs of the first type and SiC-NTs of the third type have not yet been discovered; only nanotubular fibers of the second type were obtained experimentally.
Starting Page	3
Ending Page	15
Page Count	13
File Format	PDF
ISSN	00405760
Journal	Theoretical and Experimental Chemistry
Volume Number	42
Issue Number	1
e-ISSN	1573935X
Language	English
Publisher	Kluwer Academic Publishers-Consultants Bureau
Publisher Date	2006-01-01
Publisher Place	New York
Access Restriction	One Nation One Subscription (ONOS)
Subject Keyword	nanotube nanofiber nanotubular fiber silicon carbide SiC Chemistry/Food Science
Content Type	Text
Resource Type	Article
Subject	Chemistry

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